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http://hdl.handle.net/10261/343952
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dc.contributor.author | Escobar, Javier Enrique | es_ES |
dc.contributor.author | Molina Fernández, Juan | es_ES |
dc.contributor.author | Gil-Santos, Eduardo | es_ES |
dc.contributor.author | Ruz Martínez, José Jaime | es_ES |
dc.contributor.author | Malvar, Óscar | es_ES |
dc.contributor.author | Kosaka, Priscila M. | es_ES |
dc.contributor.author | Tamayo de Miguel, Francisco Javier | es_ES |
dc.contributor.author | San Paulo, Álvaro | es_ES |
dc.contributor.author | Calleja, Montserrat | es_ES |
dc.date.accessioned | 2024-01-26T11:24:22Z | - |
dc.date.available | 2024-01-26T11:24:22Z | - |
dc.date.issued | 2023-10-30 | - |
dc.identifier.citation | ACS Nano 17(21): 21044–21055 (2023) | es_ES |
dc.identifier.issn | 1936-0851 | - |
dc.identifier.uri | http://hdl.handle.net/10261/343952 | - |
dc.description.abstract | Open nanofluidic systems, where liquids flow along the outer surface of nanoscale structures, provide otherwise unfeasible capabilities for extremely miniaturized liquid handling applications. A critical step toward fully functional applications is to obtain quantitative mass flow control. We demonstrate the application of nanomechanical sensing for this purpose by integrating voltage-driven liquid flow along nanowire open channels with mass detection based on flexural resonators. This approach is validated by assembling the nanowires with microcantilever resonators, enabling high-precision control of larger flows, and by using the nanowires as resonators themselves, allowing extremely small liquid volume handling. Both implementations are demonstrated by characterizing voltage-driven flow of ionic liquids along the surface of the nanowires. We find a voltage range where mass flow rate follows a nonlinear monotonic increase, establishing a steady flow regime for which we show mass flow control at rates from below 1 ag/s to above 100 fg/s and precise liquid handling down to the zeptoliter scale. The observed behavior of mass flow rate is consistent with a voltage-induced transition from static wetting to dynamic spreading as the mechanism underlying liquid transport along the nanowires. | es_ES |
dc.description.sponsorship | This work was supported by European Research Council through ERC CoG Grant 681275; project PID2021- 128395OB-I00 funded by MCIN/AEI/10.13039/ 501100011033/FEDER, UE; Projects PDC2022-133944-I00 and PLEC2021-007892 funded by MCIN/AEI/10.13039/ 501100011033 and European Union “NextGenerationEU”/ PRTR; Project Y2020/BIO-65194 funded by Comunidad de Madrid; Grant RYC-2019-026626-I funded by MCIN; Project AES (DTS21/00136) funded by ISCIII/Unión Europea/ FEDER. We acknowledge the service from the Micro and Nanofabrication Laboratory at IMN-CNM, funded by the Comunidad de Madrid (Project S2018/NMT-4291 TEC2- SPACE) and by MINECO (project CSIC13-4E-1794 with support from FEDER, FSE). | es_ES |
dc.format | application/pdf | es_ES |
dc.language.iso | eng | es_ES |
dc.publisher | American Chemical Society | es_ES |
dc.relation | info:eu-repo/grantAgreement/EC/H2020/681275 | es_ES |
dc.relation | info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2021-2023/PID2021-128395OB-I00/ES/ESPECTROMETRIA NANOMECANICA DE AEROSOLES PARA DETECCION DE VIRUS EN EL AIRE/ | es_ES |
dc.relation | info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2021-2023/PDC2022-133944-I00/ES/ANALISIS DE LA VIABILIDAD TECNICA DE LA DETECCION DE VIRUS AEROTRANSPORTADOS MEDIANTE ESPECTROSCOPIA NANOMECANCIA/ | es_ES |
dc.relation | info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020/PLEC2021-007892/ES/Plataforma (Oncodeeplasm) para inmunoensayos optoplasmónicos ultrasensibles para la detección temprana del cáncer de mama basada en biomarcadores de proteínas en la región profunda del proteoma sanguíneo/ | es_ES |
dc.relation | Y2020/BIO-65194 | es_ES |
dc.relation | info:eu-repo/grantAgreement/AEI//RYC-2019-026626-I | es_ES |
dc.relation | S2018/NMT-4291/TEC2- SPACE | es_ES |
dc.relation | info:eu-repo/grantAgreement/MINECO//CSIC13-4E-1794/ES/Microscopio Electrónico de Barrido de Emisión de Campo (FE-SEM)/ | es_ES |
dc.relation.isversionof | Publisher's version | es_ES |
dc.relation.isbasedon | Escobar, Javier Enrique; Molina Fernández, Juan; Gil-Santos, Eduardo; Ruz Martínez, José Jaime; Malvar, Óscar; Kosaka, Priscila M.; Tamayo de Miguel, Francisco Javier; San Paulo, Álvaro; Calleja, Montserrat; 2023; Supporting Information Nanomechanical Sensing for Mass Flow Control in Nanowire-Based Open Nanofluidic Systems[Dataset]; ACS Nano; https://doi.org/10.1021/acsnano.3c04020 | - |
dc.rights | openAccess | es_ES |
dc.subject | Semiconductor nanowires | es_ES |
dc.subject | Silicon nanowires | es_ES |
dc.subject | Nanoelectromechanical systems (NEMS) | es_ES |
dc.subject | Nanomechanical resonators | es_ES |
dc.subject | Nanofluidics | es_ES |
dc.subject | Open fluidics | es_ES |
dc.subject | Ionic liquids | es_ES |
dc.title | Nanomechanical Sensing for Mass Flow Control in Nanowire-Based Open Nanofluidic Systems | es_ES |
dc.type | artículo | es_ES |
dc.identifier.doi | 10.1021/acsnano.3c04020 | - |
dc.description.peerreviewed | Peer reviewed | es_ES |
dc.relation.publisherversion | https://doi.org/10.1021/acsnano.3c04020 | es_ES |
dc.identifier.e-issn | 1936-086X | - |
dc.rights.license | https://creativecommons.org/licenses/by-nc-nd/4.0/ | es_ES |
dc.contributor.funder | European Research Council | es_ES |
dc.contributor.funder | European Commission | es_ES |
dc.contributor.funder | Agencia Estatal de Investigación (España) | es_ES |
dc.contributor.funder | Ministerio de Ciencia e Innovación (España) | es_ES |
dc.contributor.funder | Comunidad de Madrid | es_ES |
dc.contributor.funder | Instituto de Salud Carlos III | es_ES |
dc.contributor.funder | Ministerio de Economía y Competitividad (España) | es_ES |
dc.relation.csic | Sí | es_ES |
oprm.item.hasRevision | no ko 0 false | * |
dc.identifier.funder | http://dx.doi.org/10.13039/501100011033 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/100012818 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100000780 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100000781 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100004587 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100004837 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100003329 | es_ES |
dc.type.coar | http://purl.org/coar/resource_type/c_6501 | es_ES |
item.cerifentitytype | Publications | - |
item.languageiso639-1 | en | - |
item.openairecristype | http://purl.org/coar/resource_type/c_18cf | - |
item.grantfulltext | open | - |
item.fulltext | With Fulltext | - |
item.openairetype | artículo | - |
Aparece en las colecciones: | (IMN-CNM) Artículos |
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