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http://hdl.handle.net/10261/342688
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dc.contributor.author | Martínez Berges, Isabel | es_ES |
dc.contributor.author | Romano, M. C. | es_ES |
dc.contributor.author | Fernández García, José Ramón | es_ES |
dc.contributor.author | Chiesa, Paolo | es_ES |
dc.contributor.author | Murillo Villuendas, Ramón | es_ES |
dc.contributor.author | Abanades García, Juan Carlos | es_ES |
dc.date.accessioned | 2024-01-17T18:50:05Z | - |
dc.date.available | 2024-01-17T18:50:05Z | - |
dc.date.issued | 2013-10-17 | - |
dc.identifier | doi: 10.1016/j.apenergy.2013.09.026 | - |
dc.identifier | issn: 0306-2619 | - |
dc.identifier | e-issn: 1872-9118 | - |
dc.identifier.citation | Applied Energy 114: 192-208 (2014) | es_ES |
dc.identifier.uri | http://hdl.handle.net/10261/342688 | - |
dc.description | 8 figures, 4 tables.-- © 2013. This manuscript version is made available under the CC-BY-NC-ND 4.0 license https://creativecommons.org/licenses/by-nc-nd/4.0/ | es_ES |
dc.description.abstract | A detailed and comprehensive design of a H2 production plant based on a novel Ca/Cu chemical looping process is presented in this work. This H2 production process is based on the sorption-enhanced reforming concept using natural gas together with a CaO/CaCO3 chemical loop. A second Cu/CuO loop is incorporated to supply energy for the calcination of the CaCO3 via the reduction of CuO with a fuel gas. A comprehensive energy integration description of the different gas streams available in the plant is provided to allow a thermodynamic assessment of the process and to highlight its advantages and drawbacks. Hydrogen equivalent efficiencies of up to 77% are feasible with this novel Ca/Cu looping process, using an active reforming catalyst based on Pt, high oxidation temperatures and moderate gas velocities in the fixed bed system, which are around 6% points above the efficiency of a reference H2 production plant based on conventional steam reforming including CO2 capture with MDEA. Non-converted carbon compounds in the reforming stage are removed as CO2 in the calcination stage of the Ca/Cu looping process, which will be compressed and sent for storage. Carbon capture efficiencies of around 94% can be obtained with this Ca/Cu looping process, which are significantly higher than those obtained in the reference plant that uses MDEA absorption (around 85%). Additional advantages, such as its compact design and the use of cheaper materials compared to other commercial processes for H2 production with CO2 capture, confirm the potential of the Ca/Cu looping process as a pre-combustion CO2 capture technology for H2 production. | es_ES |
dc.description.sponsorship | This work is supported by the R+D Spanish National Program from the Spanish Ministry of Economy and Competitiveness under Project ENE2012-37936-C02-01 and from CSIC 201280E017. Financial support for the PhD of I. Martínez is provided by the FPU programme of the Spanish Ministry of Education (AP2009- 3575), and funding to carry out this work has been provided by the Europe programme of the CAI. | es_ES |
dc.language | eng | - |
dc.language.iso | eng | es_ES |
dc.publisher | Elsevier | es_ES |
dc.relation | info:eu-repo/grantAgreement/MINECO//ENE2012-37936-C02-01 | es_ES |
dc.relation.isversionof | Postprint | es_ES |
dc.rights | openAccess | es_ES |
dc.subject | Ca/Cu looping process | es_ES |
dc.subject | CO2 capture | es_ES |
dc.subject | Pressurized H2 production | es_ES |
dc.title | Process design of a hydrogen production plant from natural gas with CO2 capture based on a novel Ca/Cu chemical loop | es_ES |
dc.type | artículo | es_ES |
dc.description.peerreviewed | Peer reviewed | es_ES |
dc.relation.publisherversion | http://dx.doi.org/10.1016/j.apenergy.2013.09.026 | es_ES |
dc.date.updated | 2024-01-17T18:50:05Z | - |
dc.rights.license | https://creativecommons.org/licenses/by-nc-nd/4.0/deed.es | es_ES |
dc.contributor.funder | Ministerio de Economía y Competitividad (España) | es_ES |
dc.contributor.funder | Consejo Superior de Investigaciones Científicas (España) | es_ES |
dc.contributor.funder | Ministerio de Educación (España) | es_ES |
dc.contributor.funder | European Commission | es_ES |
dc.relation.csic | Sí | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100003339 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100000780 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100003329 | es_ES |
dc.contributor.orcid | Martínez Berges, Isabel [0000-0002-2364-463X] | es_ES |
dc.contributor.orcid | Romano, M. C. [0000-0003-0213-2245] | es_ES |
dc.contributor.orcid | Fernández García, José Ramón [0000-0001-9801-7043] | es_ES |
dc.contributor.orcid | Chiesa, Paolo [0000-0003-2006-0230] | es_ES |
dc.contributor.orcid | Murillo Villuendas, Ramón [0000-0002-0299-506X] | es_ES |
dc.contributor.orcid | Abanades García, Juan Carlos [0000-0003-1711-6993] | es_ES |
dc.type.coar | http://purl.org/coar/resource_type/c_6501 | es_ES |
item.grantfulltext | open | - |
item.fulltext | With Fulltext | - |
item.openairecristype | http://purl.org/coar/resource_type/c_18cf | - |
item.languageiso639-1 | en | - |
item.cerifentitytype | Publications | - |
item.openairetype | artículo | - |
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Process_design_H2_prod._plant_Romano.pdf | 1,43 MB | Adobe PDF | Visualizar/Abrir |
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