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Título: | A 3D extra-large-pore zeolite enabled by 1D-to-3Dtopotactic condensation of a chain silicate |
Autor: | Li, Jian CSIC ORCID; Gao, Zihao Rei; Lin, Qing-Fang; Liu, Chenxu; Gao, Fangxin; Lin, Cong; Zhang, Siyao; Deng, Hua; Mayoral, Álvaro CSIC ORCID; Fan, Wei; Luo, Song; Chen, Xiaobo; He, Hong; Camblor, Miguel Ángel CSIC ORCID ; Chen, Fei-Jian; Yu, Jihong | Palabras clave: | Zeolites Silicates |
Fecha de publicación: | 20-ene-2023 | Citación: | Science 379: 283-287 (2023) | Resumen: | Zeolites are microporous silicates with a large variety of applications as catalysts, adsorbents, and cationexchangers. Stable silica-based zeolites with increased porosity are in demand to allow adsorption andprocessing of large molecules but challenge our synthetic ability. We report a new, highly stable pure silicazeolite called ZEO-3, which has a multidimensional, interconnected system of extra-large pores open throughwindows made by 16 and 14 silicate tetrahedra, the least dense polymorph of silica known so far. This zeolitewas formed by an unprecedented one-dimensional to three-dimensional (1D-to-3D) topotactic condensationof a chain silicate. With a specific surface area of more than 1000 square meters per gram, ZEO-3 showed ahigh performance for volatile organic compound abatement and recovery compared with other zeolites andmetal-organic frameworks. | Descripción: | Anyone can access the published paper FREE OF CHARGE by clicking on this link: [Cualquier persona puede acceder al documento publicado de forma GRATUITA, accediendo a través del enlace] | Versión del editor: | https://www.science.org/stoken/author-tokens/ST-242/full https://www.science.org/doi/epdf/10.1126/science.ade1771 |
URI: | http://hdl.handle.net/10261/287377 | DOI: | 10.1126/science.ade1771 | ISSN: | 0036-8075 | E-ISSN: | 1095-9203 |
Aparece en las colecciones: | (ICMM) Artículos (INMA) Artículos |
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Li_A_3D_extra_Science_20_1_23_Postprint.pdf | Artículo principal-Vs Postprint | 3,87 MB | Adobe PDF | Visualizar/Abrir |
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