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dc.contributor.author | Khobotov-Bakishev, Akim | es_ES |
dc.contributor.author | Baeckmann, Cornelia von | es_ES |
dc.contributor.author | Ortín-Rubio, Borja | es_ES |
dc.contributor.author | Hernández-López, Laura | es_ES |
dc.contributor.author | Cortés Martínez, Alba | es_ES |
dc.contributor.author | Martínez Esaín, Jordi | es_ES |
dc.contributor.author | Gándara Barragán, Felipe | es_ES |
dc.contributor.author | Juanhuix, Judith | es_ES |
dc.contributor.author | Platero Prats, Ana E. | es_ES |
dc.contributor.author | Faraudo, Jordi | es_ES |
dc.contributor.author | Carné-Sánchez, Arnau | es_ES |
dc.contributor.author | Maspoch, Daniel | es_ES |
dc.date.accessioned | 2022-11-22T08:57:14Z | - |
dc.date.available | 2022-11-22T08:57:14Z | - |
dc.date.issued | 2022-08-31 | - |
dc.identifier.citation | Journal of the American Chemical Society 144(34): 15745-15753 (2022) | es_ES |
dc.identifier.issn | 0002-7863 | - |
dc.identifier.uri | http://hdl.handle.net/10261/283434 | - |
dc.description.abstract | Metal-organic frameworks (MOFs) assembled from multiple building blocks exhibit greater chemical complexity and superior functionality in practical applications. Herein, we report a new approach based on using prefabricated cavities to design isoreticular multicomponent MOFs from a known parent MOF. We demonstrate this concept with the formation of multicomponent HKUST-1 analogues, using a prefabricated cavity that comprises a cuboctahedral Rh(II) metal-organic polyhedron functionalized with 24 carboxylic acid groups. The cavities are reticulated in three dimensions via Cu(II)-paddlewheel clusters and (functionalized) 1,3,5-benzenetricarboxylate linkers to form three- and four-component HKUST-1 analogues. | es_ES |
dc.description.sponsorship | This work was supported by the Spanish MINECO (project RTI2018-095622-B-I00), the Catalan AGAUR (project 2017 SGR 238), the CERCA Program/Generalitat de Catalunya, and the MCIN/AEI/10.13039/501100011033 and by the European Union “NextGenerationEU”/PRTR (EUR2020-112294). We also thank CESGA Supercomputing center for technical support and computer time at the supercomputer Finisterrae III. ICN2 and ICMAB are supported by the Severo Ochoa program from the Spanish MINECO (grants SEV-2017-0706 and CEX2019-000917-S). The project that gave rise to these results received the support of a fellowship (LCF/BQ/PR20/11770011) from “la Caixa” Foundation (ID 100010434). A.E.P.-P. acknowledges a Ramón y Cajal fellowship (RYC2018-024328-I). With funding from the Spanish government through the ‘Severo Ochoa Centre of Excellence’ accreditation (CEX2019-000917-S). | es_ES |
dc.format | application/pdf | es_ES |
dc.language.iso | eng | es_ES |
dc.publisher | American Chemical Society | es_ES |
dc.relation | info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020/RTI2018-095622-B-I00/ES/POLIEDROS METAL-ORGANICOS COMO PARTICULAS POROSAS SUB-5 NM PARA EL DESARROLLO DE NUEVOS ADSORBENTES Y SISTEMAS DE LIBERACION/ | es_ES |
dc.relation | info:eu-repo/grantAgreement/AEI//RYC2018-024328-I | es_ES |
dc.relation | info:eu-repo/grantAgreement/MINECO/Plan Estatal de Investigación Científica y Técnica y de Innovación 2013-2016/SEV-2015-0496 | es_ES |
dc.relation | info:eu-repo/grantAgreement/MICIU/Plan Estatal de investigación Científica y Técnica y de Innovación 2017-2020/CEX2019-000917-S | es_ES |
dc.relation | info:eu-repo/grantAgreement/AEI//SEV-2017-0706 | es_ES |
dc.relation.ispartof | Journal of the American Chemical Society | es_ES |
dc.relation.isversionof | Publisher's version | es_ES |
dc.relation.isbasedon | Khobotov-Bakishev, Akim; Baeckmann, Cornelia von; Ortín-Rubio, Borja; Hernández-López, Laura; Cortés Martínez, Alba; Martínez Esaín, Jordi; Gándara Barragán, Felipe; Juanhuix, Judith; Platero Prats, Ana E.; Faraudo, Jordi; Carné-Sánchez, Arnau; Maspoch, Daniel; 2022; Multicomponent, Functionalized HKUST‑1 Analogues Assembled via Reticulation of Prefabricated Metal–Organic Polyhedral Cavities [Dataset]; Figshare; https://doi.org/10.1021/jacs.2c06131.s001 | - |
dc.rights | openAccess | es_ES |
dc.title | Multicomponent, functionalized HKUST-1 analogues assembled via reticulation of prefabricated metal-organic polyhedral cavities | es_ES |
dc.type | artículo | es_ES |
dc.identifier.doi | 10.1021/jacs.2c06131 | - |
dc.description.peerreviewed | Peer reviewed | es_ES |
dc.relation.publisherversion | http://dx.doi.org/10.1021/jacs.2c06131 | es_ES |
dc.rights.license | https://creativecommons.org/licenses/by/4.0/ | es_ES |
dc.contributor.funder | Ministerio de Ciencia, Innovación y Universidades (España) | es_ES |
dc.contributor.funder | Generalitat de Catalunya | es_ES |
dc.contributor.funder | European Commission | es_ES |
dc.contributor.funder | Ministerio de Economía y Competitividad (España) | es_ES |
dc.contributor.funder | Fundación la Caixa | es_ES |
dc.contributor.funder | Agencia Estatal de Investigación (España) | es_ES |
dc.relation.csic | Sí | es_ES |
oprm.item.hasRevision | no ko 0 false | * |
dc.identifier.funder | http://dx.doi.org/10.13039/501100002809 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100000780 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100003329 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100011033 | es_ES |
dc.contributor.orcid | Ortín Rubio, Borja [0000-0002-0533-3635] | es_ES |
dc.contributor.orcid | Martínez Esaín, Jordi [0000-0002-8420-8559] | es_ES |
dc.contributor.orcid | Gándara, Felipe [0000-0002-1671-6260] | es_ES |
dc.contributor.orcid | Juanhuix, Judith [0000-0003-3728-8215] | es_ES |
dc.contributor.orcid | Platero Prats, Ana E. [0000-0002-2248-2739] | es_ES |
dc.contributor.orcid | Faraudo, Jordi [0000-0002-6315-4993] | es_ES |
dc.contributor.orcid | Carné Sánchez, Arnau [0000-0002-8569-6208] | es_ES |
dc.contributor.orcid | Maspoch, Daniel [0000-0003-1325-9161] | es_ES |
dc.identifier.pmid | 35973046 | - |
dc.identifier.scopus | 2-s2.0-85136481275 | - |
dc.identifier.url | https://api.elsevier.com/content/abstract/scopus_id/85136481275 | - |
dc.type.coar | http://purl.org/coar/resource_type/c_6501 | es_ES |
item.cerifentitytype | Publications | - |
item.languageiso639-1 | en | - |
item.openairecristype | http://purl.org/coar/resource_type/c_18cf | - |
item.grantfulltext | open | - |
item.fulltext | With Fulltext | - |
item.openairetype | artículo | - |
Aparece en las colecciones: | (ICMAB) Artículos (CIN2) Artículos |
Ficheros en este ítem:
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Khobotov_JACS_2022_editorial.pdf | Artículo principal | 7,02 MB | Adobe PDF | Visualizar/Abrir |
Khobotov_JACS_2022_suppl_editorial.pdf | Información complementaria | 58,7 MB | Adobe PDF | Visualizar/Abrir |
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