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Título: | Synthesis and Characterization of Ethylenedithio-MPTTF-PTM Radical Dyad as a Potential Neutral Radical Conductor |
Autor: | Souto Salom, Manuel; Bendixen, Dan; Jensen, Morten; Díez Cabanes, Valentín; Cornil, Jérôme; Jeppesen, Jan O.; Ratera, Immaculada; Rovira, Concepció CSIC ORCID; Veciana, Jaume CSIC ORCID CVN | Palabras clave: | Neutral organic radical Perchlorotriphenylmethyl radical Tetrathiafulvalene Donor-acceptor |
Fecha de publicación: | 16-dic-2016 | Editor: | Multidisciplinary Digital Publishing Institute | Citación: | Magnetochemistry 2(4): 46 (2016) | Resumen: | During the last years there has been a high interest in the development of new purely-organic single-component conductors. Very recently, we have reported a new neutral radical conductor based on the perchlorotriphenylmethyl (PTM) radical moiety linked to a monopyrrolotetrathiafulvalene (MPTTF) unit by a π-conjugated bridge (1) that behaves as a semiconductor under high pressure. With the aim of developing a new material with improved conducting properties, we have designed and synthesized the radical dyad 2 which was functionalized with an ethylenedithio (EDT) group in order to improve the intermolecular interactions of the tetrathiafulvalene (TTF) subunits. The physical properties of the new radical dyad 2 were studied in detail in solution to further analyze its electronic structure. | Versión del editor: | http://dx.doi.org/10.3390/magnetochemistry2040046 | URI: | http://hdl.handle.net/10261/150766 | DOI: | 10.3390/magnetochemistry2040046 | E-ISSN: | 2312-7481 |
Aparece en las colecciones: | (ICMAB) Artículos |
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Souto_Magnetochem_2016_editorial.pdf | Artículo principal | 2,89 MB | Adobe PDF | Visualizar/Abrir |
Souto_Magnetochem_2016_suppl_editorial.pdf | Información complementaria | 1,42 MB | Adobe PDF | Visualizar/Abrir |
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