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Título: | Pt-Ni contact engineering in carbon nitride based photocatalysts for hydrogen production |
Autor: | Sayago-Carro, Rocío; Piqueras-Pérez, Pablo; Du, Ruifeng; Li, Junshan; Yu, Jing; Arbiol, Jordi CSIC ORCID CVN; Kubacka, Anna CSIC ORCID; Cabot, Andreu; Fernández-García, Marcos CSIC ORCID | Palabras clave: | Photocatalysis Quantum efficiency Hydrogen Pt-Ni alloy Carbon nitride Methanol Nanosheet |
Fecha de publicación: | 2023 | Editor: | Elsevier | Citación: | Journal of Environmental Chemical Engineering 11(5): 110921 (2023) | Resumen: | The effect of a binary PtNi co-catalyst supported on graphitic carbon nitride nanosheets is studied in the photo-production of hydrogen from methanol:water mixtures. The physicochemical analysis provides evidence that the carbon nitride support allows the formation of highly dispersed PtNi nanoparticles with an average composition of Pt 85 % Ni 15 %. The binary system outperforms the monometallic Pt and Ni counterparts and renders an extraordinary quantum efficiency of 8.8 % for hydrogen photo-production. The formation of a PtNi alloy, with a Pt-enriched surface and electronic properties influenced by the heterometallic contact, provides high and stable activity, mostly as a consequence of the effects that the co-catalyst exerts on the charge carrier handling capability of the solid. | Versión del editor: | https://doi.org/10.1016/j.jece.2023.110921 | URI: | http://hdl.handle.net/10261/347160 | DOI: | 10.1016/j.jece.2023.110921 | E-ISSN: | 2213-3437 |
Aparece en las colecciones: | (CIN2) Artículos (ICP) Artículos |
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ptniproduct.pdf | 5,07 MB | Adobe PDF | Visualizar/Abrir |
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