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http://hdl.handle.net/10261/284586
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dc.contributor.author | Yu, Jiahao | es_ES |
dc.contributor.author | Garcés-Pineda, Felipe A. | es_ES |
dc.contributor.author | González-Cobos, Jesús | es_ES |
dc.contributor.author | Peña-Díaz, Marina | es_ES |
dc.contributor.author | Rogero, Celia | es_ES |
dc.contributor.author | Giménez, Sixto | es_ES |
dc.contributor.author | Spadaro, Maria Chiara | es_ES |
dc.contributor.author | Arbiol, Jordi | es_ES |
dc.contributor.author | Barja, Sara | es_ES |
dc.contributor.author | Galán-Mascarós, José Ramón | es_ES |
dc.date.accessioned | 2022-12-09T09:03:00Z | - |
dc.date.available | 2022-12-09T09:03:00Z | - |
dc.date.issued | 2022 | - |
dc.identifier.citation | Nature Communications 13: 4341 (2022) | es_ES |
dc.identifier.uri | http://hdl.handle.net/10261/284586 | - |
dc.description.abstract | Earth-abundant electrocatalysts for the oxygen evolution reaction (OER) able to work in acidic working conditions are elusive. While many first-row transition metal oxides are competitive in alkaline media, most of them just dissolve or become inactive at high proton concentrations where hydrogen evolution is preferred. Only noble-metal catalysts, such as IrO2, are fast and stable enough in acidic media. Herein, we report the excellent activity and long-term stability of Co3O4-based anodes in 1 M H2SO4 (pH 0.1) when processed in a partially hydrophobic carbon-based protecting matrix. These Co3O4@C composites reliably drive O2 evolution a 10 mA cm–2 current density for >40 h without appearance of performance fatigue, successfully passing benchmarking protocols without incorporating noble metals. Our strategy opens an alternative venue towards fast, energy efficient acid-media water oxidation electrodes. | es_ES |
dc.description.sponsorship | The authors thank the support from projects RED2018-102459-T, RTI2018-095618-B-I00, PID2020-116093RB-C41,C43&C44, PID2019-107338RB-C63 and PID2020-114252GB-I00 funded by MCIN/AEI/10.13039/501100011033/ and by “ERDF A way of making Europe”; the Generalitat de Catalunya (2017-SGR-1406 and 2017-SGR-327), and the Basque Government (grant IT1591-22). J.Y. thanks the China Scholarship Council (CSC) for predoctoral fellowships (File No. 201806270234). S.B. acknowledges Grant RYC-2017-21931 funded by MCIN/AEI/ 10.13039/501100011033 and by ESF Investing in your future, and UPV/EHU project EHUrOPE19/01 and IKERBASQUE, Basque Foundation for Science. ICIQ and ICN2 are supported by the Ministerio de Ciencia e Innovación through the Severo Ochoa Excellence Accreditations CEX2019-000925-S (MIC/AEI) and SEV-2017-0706; and by the CERCA Programme/Generalitat de Catalunya. M.C.S. has received funding from the European Union’s Horizon 2020 research and innovation programme under Marie Skodowska-Curie grant 754510 (PROBIST) and the Severo Ochoa programme. M.C.S. has received funding from the postdoctoral fellowship Juan de la Cierva Incorporation from MICINN (JCI-2019) and the Severo Ochoa programme. M.P.D. acknowledges funding for a Ph.D. fellowship from the MPC Foundation. | es_ES |
dc.format | application/pdf | es_ES |
dc.language.iso | eng | es_ES |
dc.publisher | Springer Nature | es_ES |
dc.relation | info:eu-repo/grantAgreement/AEI//RED2018-102459-T | es_ES |
dc.relation | info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020/RTI2018-095618-B-I00/ES/NUEVAS ESTRATEGIAS (FOTO)ELECTROQUIMICAS PARA LA TRANSFORMACION DE ENERGIAS RENOVABLES EN VECTORES ENERGETICOS SOSTENIBLES/ | es_ES |
dc.relation | info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020/PID2020-116093RB-C41/ES/DESARROLLO DE SISTEMAS ELECTROCATALITICOS INTEGRADOS PARA LA SINTESIS DE PRODUCTOS QUIMICOS DE ALTO VALOR AÑADIDO/ | es_ES |
dc.relation | info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020/PID2020-116093RB-C43/ES/NANOSCOPIAS ELECTRONICAS AVANZADAS APLICADAS A LA INVESTIGACION Y MEJORA DE ELECTROCATALITICOS PARA LA GENERACION DE COMBUSTIBLES SOSTENIBLES Y PRODUCTOS DE ALTO VALOR AÑADIDO/ | es_ES |
dc.relation | info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020/PID2020-116093RB-C44/ES/ESTUDIO DE LAS RELACIONES ESTRUCTURA-FUNCION EN CATALIZADOR MODELO PARA LA GENERACION LIMPIA DE PRODUCTOS QUIMICOS DE ALTO VALOR AÑADIDO./ | es_ES |
dc.relation | info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020/PID2019-107338RB-C63/ES/TRANSFERENCIA DE SISTEMAS MOLECULARES FUNCIONALES A SUPERFICIES NO METALICAS/ | es_ES |
dc.relation | info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020/PID2020-114252GB-I00/ES/ESPINTRONICA Y ESPIN-ORBITRONICA EN NANOESTRUCTURAS HIBRIDAS: DE LAS TECNOLOGIAS CLASICAS A LAS CUANTICAS./ | es_ES |
dc.relation | info:eu-repo/grantAgreement/AEI//RYC-2017-21931 | es_ES |
dc.relation | info:eu-repo/grantAgreement/AEI//CEX2019-000925-S | es_ES |
dc.relation | info:eu-repo/grantAgreement/AEI//SEV-2017-0706 | es_ES |
dc.relation | info:eu-repo/grantAgreement/EC/H2020/754510 | es_ES |
dc.relation.isversionof | Publisher's version | es_ES |
dc.relation.isbasedon | The underlying dataset has been published as supplementary material of the article in the publisher platform at DOI 10.1038/s41467-022-32024-6 | - |
dc.relation.isreferencedby | Yu, Jiahao; Garcés-Pineda, Felipe A.; González-Cobos, Jesús; Peña-Díaz, Marina; Rogero, Celia; Giménez, Sixto; Spadaro, Maria Chiara; Arbiol, Jordi; Barja, Sara; Galán-Mascarós, José Ramón. Author Correction: Sustainable oxygen evolution electrocatalysis in aqueous 1 M H2SO4 with earth abundant nanostructured Co3O4. https://doi.org/10.1038/s41467-022-32399-6. http://hdl.handle.net/10261/297099 | - |
dc.rights | openAccess | es_ES |
dc.title | Sustainable oxygen evolution electrocatalysis in aqueous 1 MH2SO4 with earth abundant nanostructured Co3O4 | es_ES |
dc.type | artículo | es_ES |
dc.identifier.doi | 10.1038/s41467-022-32024-6 | - |
dc.description.peerreviewed | Peer reviewed | es_ES |
dc.relation.publisherversion | https://doi.org/10.1038/s41467-022-32024-6 | es_ES |
dc.identifier.e-issn | 2041-1723 | - |
dc.rights.license | http://creativecommons.org/licenses/by/4.0/ | es_ES |
dc.contributor.funder | Ministerio de Ciencia, Innovación y Universidades (España) | es_ES |
dc.contributor.funder | Agencia Estatal de Investigación (España) | es_ES |
dc.contributor.funder | Generalitat de Catalunya | es_ES |
dc.contributor.funder | European Commission | es_ES |
dc.contributor.funder | Universidad del País Vasco | es_ES |
dc.contributor.funder | Eusko Jaurlaritza | es_ES |
dc.contributor.funder | China Scholarship Council | es_ES |
dc.relation.csic | Sí | es_ES |
oprm.item.hasRevision | no ko 0 false | * |
dc.identifier.funder | http://dx.doi.org/10.13039/501100011033 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100004543 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100000780 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100003086 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100002809 | es_ES |
dc.type.coar | http://purl.org/coar/resource_type/c_6501 | es_ES |
item.grantfulltext | open | - |
item.openairecristype | http://purl.org/coar/resource_type/c_18cf | - |
item.fulltext | With Fulltext | - |
item.cerifentitytype | Publications | - |
item.languageiso639-1 | en | - |
item.openairetype | artículo | - |
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