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Título: | A highly versatile polymer network based on liquid crystalline dendrimers |
Autor: | Cervera-Procas, Ramón CSIC; Serrano, José Luis CSIC ORCID; Omenat, Ana CSIC ORCID | Palabras clave: | Dendrimer Dye encapsulation Polymer networks Responsive materials Liquid crystal Microporous structure |
Fecha de publicación: | 2021 | Editor: | Multidisciplinary Digital Publishing Institute | Citación: | International Journal of Molecular Sciences 22(11): 5740 (2021) | Resumen: | Highly functional macromolecules with a well-defined architecture are the key to designing efficient and smart materials, and these polymeric systems can be tailored for specific applications in a diverse range of fields. Herein, the formation of a new liquid crystalline polymeric network based on the crosslinking of dendrimeric entities by the CuI-catalyzed variant of the Huisgen 1,3-dipolar cycloaddition of azides and alkynes to afford 1,2,3-triazoles is reported. The polymeric material obtained in this way is easy to process and exhibits a variety of properties, which include mesomorphism, viscoelastic behavior, and thermal contraction. The porous microstructure of the polymer network determines its capability to absorb solvent molecules and to encapsulate small molecules, like organic dyes, which can be released easily afterwards. Moreover, all these properties may be easily tuned by modifying the chemical structure of the constituent dendrimers, which makes this system a very interesting one for a number of applications. | Descripción: | This article belongs to the Special Issue Nanostructured Materials Based on Liquid Crystals. | Versión del editor: | https://doi.org/10.3390/ijms22115740 | URI: | http://hdl.handle.net/10261/265433 | DOI: | https://doi.org/10.3390/ijms22115740 | E-ISSN: | 1422-0067 |
Aparece en las colecciones: | (INMA) Artículos |
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ahighdendrim.pdf | 3,28 MB | Adobe PDF | Visualizar/Abrir |
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