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http://hdl.handle.net/10261/188701
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Campo DC | Valor | Lengua/Idioma |
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dc.contributor.author | Sánchez, Carlos | es_ES |
dc.contributor.author | Nicolaï, Adrien | es_ES |
dc.contributor.author | Rossel, Frédéric | es_ES |
dc.contributor.author | Cai, Jinming | es_ES |
dc.contributor.author | Liu, Junzhi | es_ES |
dc.contributor.author | Feng, Xinliang | es_ES |
dc.contributor.author | Müllen, Klaus | es_ES |
dc.contributor.author | Ruffieux, Pascal | es_ES |
dc.contributor.author | Fasel, Román | es_ES |
dc.contributor.author | Meunier, Vincent | es_ES |
dc.date.accessioned | 2019-08-21T09:11:39Z | - |
dc.date.available | 2019-08-21T09:11:39Z | - |
dc.date.issued | 2017-12-06 | - |
dc.identifier | doi: 10.1021/jacs.7b10026 | - |
dc.identifier | issn: 0002-7863 | - |
dc.identifier | e-issn: 1520-5126 | - |
dc.identifier.citation | Journal of the American Chemical Society 139(48): 17617-17623 (2017) | es_ES |
dc.identifier.uri | http://hdl.handle.net/10261/188701 | - |
dc.description.abstract | We report on the surface-catalyzed formal [2+2] and [2+2+2] cycloadditions of ortho-activated tetracene species on a Ag(111) substrate under ultrahigh vacuum conditions. Three different products are obtained: tetracene dimers, trimers, and tetramers. The former results from the formation of a four-membered ring while the other two arise from cyclization into six-membered rings. These on-surface reactions have been monitored by scanning tunneling microscopy and rationalized by density functional theory calculations. Our approach, based on the reaction of ortho-dihalo precursor monomers via formal cycloadditions, establishes an additional method for the highly active field of on-surface synthesis and enables the development of novel 1D and 2D covalent carbon nanostructures. | - |
dc.description.sponsorship | We are grateful for financial support from the Swiss National Science Foundation, the Office of Naval Research BRC program, and the European Commission Graphene Flagship (No. CNECT-ICT-604391). CSS is grateful to Ministerio de Economía y Competitividad for financial support via the Juan de la Cierva Incorporación grant (IJCI-2014-19291). | - |
dc.publisher | American Chemical Society | es_ES |
dc.relation | info:eu-repo/grantAgreement/EC/FP7/604391 | - |
dc.relation | info:eu-repo/grantAgreement/MINECO/Plan Estatal de Investigación Científica y Técnica y de Innovación 2013-2016/IJCI-2014-19291 | - |
dc.rights | closedAccess | - |
dc.title | On-surface cyclization of ortho-dihalotetracenes to four- and six-membered rings | es_ES |
dc.type | artículo | es_ES |
dc.identifier.doi | 10.1021/jacs.7b10026 | - |
dc.relation.publisherversion | https://doi.org/10.1021/jacs.7b10026 | - |
dc.date.updated | 2019-08-21T09:11:39Z | - |
dc.language.rfc3066 | eng | - |
dc.contributor.funder | Swiss National Science Foundation | - |
dc.contributor.funder | Office of Naval Research (US) | - |
dc.contributor.funder | European Commission | - |
dc.contributor.funder | Ministerio de Economía y Competitividad (España) | - |
dc.relation.csic | Sí | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/100000006 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100003329 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100000780 | es_ES |
dc.type.coar | http://purl.org/coar/resource_type/c_6501 | es_ES |
item.cerifentitytype | Publications | - |
item.openairecristype | http://purl.org/coar/resource_type/c_18cf | - |
item.grantfulltext | none | - |
item.openairetype | artículo | - |
item.fulltext | No Fulltext | - |
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