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Título: | Highly dispersed Rh single atoms over graphitic carbon nitride as a robust catalyst for the hydroformylation reaction |
Autor: | Jurado, Lole; Esvan, Jerome; Luque-Álvarez, Ligia A; Bobadilla, Luis F; Odriozola, José Antonio CSIC ORCID; Posada-Pérez, Sergio; Poater, Albert; Comas-Vives, Aleix; Axet, M Rosa | Palabras clave: | Nanoparticles Evolution Insights G-C3N4 |
Tesauro UNESCO: | http://vocabularies.unesco.org/thesaurus/concept640 | Fecha de publicación: | 12-ene-2023 | Editor: | Royal Society of Chemistry (UK) | Citación: | Catalysis Science and Technology 13: 1425-1436 (2023) | Resumen: | Rhodium-catalysed hydroformylation, effective tool in bulk and fine-chemical synthesis, predominantly uses soluble metal complexes. For that reason, the metal leaching and the catalyst recycling are still the major drawbacks of this process. Single-atom catalysts have emerged as a powerful tool to combine the advantages of both homogeneous and heterogeneous catalysts. Since using an appropriate support material is key to create stable, finely dispersed, single-atom catalysts, here we show that Rh atoms anchored on graphitic carbon nitride are robust catalysts for the hydroformylation reaction of styrene. | Versión del editor: | DOI https://doi.org/10.1039/D2CY02094G | URI: | http://hdl.handle.net/10261/355523 | DOI: | 10.1039/d2cy02094g | ISSN: | 2044-4753 |
Aparece en las colecciones: | (ICMS) Artículos |
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Jurado_2023_print.pdf | Highly dispersed Rh single atoms over graphitic carbon nitride as a robust catalyst for the hydroformylation reaction | 2,65 MB | Adobe PDF | Visualizar/Abrir |
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