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Título: | Formic Acid Dehydrogenation over Ru- and Pd-Based Catalysts: Gas- vs. Liquid-Phase Reactions |
Autor: | Ruiz-López, Estela; Ribota Peláez, María; Blasco Ruz, María; Domínguez Leal, María Isabel; Martínez Tejada, Marcela; Ivanova, Svetlana CSIC ORCID; Centeno, Miguel Ángel CSIC ORCID | Palabras clave: | Hydrogen Formic acid Dehydrogenation Ru catalyst Pd catalyst Carbon nitride |
Fecha de publicación: | 4-ene-2023 | Editor: | Multidisciplinary Digital Publishing Institute | Citación: | Materials 16(2): 472 (2023) | Resumen: | Formic acid has recently been revealed to be an excellent hydrogen carrier, and interest in the development of efficient and selective catalysts towards its dehydrogenation has grown. This reaction has been widely explored using homogeneous catalysts; however, from a practical and scalable point of view, heterogeneous catalysts are usually preferred in industry. In this work, formic acid dehydrogenation reactions in both liquid- and vapor-phase conditions have been investigated using heterogeneous catalysts based on mono- or bimetallic Pd/Ru. In all of the explored conditions, the catalysts showed good catalytic activity and selectivity towards the dehydrogenation reaction, avoiding the formation of undesired CO. | Versión del editor: | https://doi.org/10.3390/ma16020472 | URI: | http://hdl.handle.net/10261/286127 | DOI: | 10.3390/ma16020472 | ISSN: | 1996-1944 |
Aparece en las colecciones: | (ICMS) Artículos |
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