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Título: | Effect of support type and crystal form of support in the catalytic gasification of old corrugated containers using Fe-based catalysts |
Autor: | Lu, Wang; Lei, Shuaishuai; Chen, Xu; Sun,Lin; Xia, Sunwen; Bartocci, Pietro CSIC ORCID; Chen, Yingquan; Yang, Haiping; Chen, Hanping | Palabras clave: | Solid waste Catalytic gasification Fe-based catalyst Support Mechanism |
Fecha de publicación: | 8-ago-2022 | Editor: | Elsevier | Citación: | Waste Management 151: 163-170 (2022) | Resumen: | Catalytic gasification of old corrugated containers with Fe-based catalysts is a promising way to produce renewable H2 along with the utilization of solid waste. In this study, the effect of support type and crystal form of support in Fe-based catalysts on the catalytic gasification of old corrugated containers was systematically investigated. The results show that, the introduction of Fe/γ-Al2O3, Fe/TiO2, Fe/SiO2, and Fe/ZSM5-30 promote H2 production. Among them, Fe/TiO2 has the highest catalytic activity on H2 yield (25.10 mmol/g) related to the formation of Fe2TiO5 solid-melt material. Fe/γ-Al2O3 shows the best H2 selectivity (46.34 %) and good H2 yield (24.19 mmol/g) due to good dispersity of Fe. Further, the order of catalytic effect on H2 selectivity is Fe/amorphous Al2O3 (51.46 %) > Fe/α-Al2O3 (46.98 %) > Fe/γ-Al2O3 (46.34 %). With the increase in cycle index, Fe/amorphous Al2O3 shows the best catalytic effect on H2 yield (25.56 mmol/g) after 11 indexes due to the formation of Al2FeO4. Fe/γ-Al2O3 shows the best stability on H2 selectivity (∼43 %) after 11 indexes. | Descripción: | 5 figures, 3 tables.-- Supplementary information available.-- © 2022. This manuscript version is made available under the CC-BY-NC-ND 4.0 license https://creativecommons.org/licenses/by-nc-nd/4.0/ | Versión del editor: | http://dx.doi.org/10.1016/j.wasman.2022.08.003 | URI: | http://hdl.handle.net/10261/280441 | DOI: | 10.1016/j.wasman.2022.08.003 | ISSN: | 0956-053X |
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