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http://hdl.handle.net/10261/176943
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Campo DC | Valor | Lengua/Idioma |
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dc.contributor.author | Sierda, Emil | - |
dc.contributor.author | Abadia, Mikel | - |
dc.contributor.author | Brede, Jens | - |
dc.contributor.author | Elsebach, Micha | - |
dc.contributor.author | Bugenhagen, Bernhard | - |
dc.contributor.author | Prosenc, Marc Heinrich | - |
dc.contributor.author | Bazarnik, Maciej | - |
dc.contributor.author | Wiesendanger, Roland | - |
dc.date.accessioned | 2019-02-28T12:39:43Z | - |
dc.date.available | 2019-02-28T12:39:43Z | - |
dc.date.issued | 2017 | - |
dc.identifier | doi: 10.1021/acsnano.7b04194 | - |
dc.identifier | e-issn: 1936-086X | - |
dc.identifier | issn: 1936-0851 | - |
dc.identifier.citation | ACS Nano 11(9): 9200-9206 (2017) | - |
dc.identifier.uri | http://hdl.handle.net/10261/176943 | - |
dc.description.abstract | Molecular spintronics is currently attracting a lot of attention due to its great advantages over traditional electronics. A variety of self-assembled molecule-based devices are under development, but studies regarding the reliability of the growth process remain rare. Here, we present a method to control the length of molecular spintronic chains and to make their terminations chemically inert, thereby suppressing uncontrolled coupling to surface defects. The temperature evolution of chain formation was followed by X-ray photoelectron spectroscopy to determine optimal growth conditions. The final structures of the chains were then studied, using scanning tunneling microscopy, as a function of oligomerization conditions. We find that short chains are readily synthesized with high yields and that long chains, even exceeding 70mers, can be realized under optimized growth parameters, albeit with reduced yields. | - |
dc.description.sponsorship | We gratefully acknowledge financial support from the Office of Naval Research via Grant No. N00014-16-1-2900, and the Deutsche Forschungsgemeinschaft via SFB668-B4. Moreover, M.A. and J.B. acknowledge funding from the Spanish MINECO under contract Nos. MAT2013-46593-C6-4-P and MAT2016-78293-C6-5-R as well as the Basque Government Grants IT621- 13 and IT-756-13. | - |
dc.publisher | American Chemical Society | - |
dc.relation | info:eu-repo/grantAgreement/MINECO/Plan Estatal de Investigación Científica y Técnica y de Innovación 2013-2016/MAT2013-46593-C6-4-P | - |
dc.relation | info:eu-repo/grantAgreement/MINECO/Plan Estatal de Investigación Científica y Técnica y de Innovación 2013-2016/MAT2016-78293-C6-5-R | - |
dc.rights | closedAccess | - |
dc.subject | Magnetic molecules | - |
dc.subject | Molecular chain growth | - |
dc.subject | On-surface chemistry | - |
dc.subject | Nanotechnology | - |
dc.subject | Molecular spintronics | - |
dc.subject | X-ray photoelectron spectroscopy | - |
dc.subject | Scanning tunneling microscopy | - |
dc.title | On-surface oligomerization of self-terminating molecular chains for the design of spintronic devices | - |
dc.type | artículo | - |
dc.identifier.doi | 10.1021/acsnano.7b04194 | - |
dc.date.updated | 2019-02-28T12:39:43Z | - |
dc.description.version | Peer Reviewed | - |
dc.language.rfc3066 | eng | - |
dc.contributor.funder | Eusko Jaurlaritza | - |
dc.contributor.funder | German Research Foundation | - |
dc.contributor.funder | Office of Naval Research (US) | - |
dc.contributor.funder | Ministerio de Economía y Competitividad (España) | - |
dc.relation.csic | Sí | - |
dc.identifier.funder | http://dx.doi.org/10.13039/501100003329 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100003086 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100001659 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/100000006 | es_ES |
dc.identifier.pmid | 28813591 | - |
dc.type.coar | http://purl.org/coar/resource_type/c_6501 | es_ES |
item.cerifentitytype | Publications | - |
item.openairecristype | http://purl.org/coar/resource_type/c_18cf | - |
item.grantfulltext | none | - |
item.fulltext | No Fulltext | - |
item.openairetype | artículo | - |
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