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Campo DC | Valor | Lengua/Idioma |
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dc.contributor.author | Canton-Vitoria, Rubén | es_ES |
dc.contributor.author | Vallan, Lorenzo | es_ES |
dc.contributor.author | Urriolabeitia, Esteban P. | es_ES |
dc.contributor.author | Benito, Ana M. | es_ES |
dc.contributor.author | Maser, Wolfgang K. | es_ES |
dc.contributor.author | Tagmatarchis, Nikos | es_ES |
dc.date.accessioned | 2018-06-18T09:06:20Z | - |
dc.date.available | 2018-06-18T09:06:20Z | - |
dc.date.issued | 2018-05-15 | - |
dc.identifier.citation | Chemistry - A European Journal 24(41): 10468-10474 (2018) | es_ES |
dc.identifier.issn | 0947-6539 | - |
dc.identifier.uri | http://hdl.handle.net/10261/166481 | - |
dc.description.abstract | We report on the preparation, characterization and photophysical and electrocatalytic properties of carbon dots (CDs)/MoS2 ensembles. Based on electrostatic interactions, ammonium functionalized MoS2, prepared upon reaction of 1,2-dithiolane tertbutyl carbamate with MoS2 followed by acidic deprotection, was coupled with CDs bearing multiple carboxylates on their periphery as derived upon microwave-assisted polycondensation of citric acid and ethylenediamine followed by alkaline treatment. Insights into electronic interactions between the two species within CDs/MoS2 emanated from absorption and photoluminescence titration assays. Efficient fluorescence quenching of CDs by MoS2 was observed and attributed to photoinduced electron/energy transfer as the decay mechanism for the transduction of the singlet excited state of CDs. Finally, the electrocatalytic performance of CDs/MoS2 was assessed towards the hydrogen evolution reaction and found superior as compared to that owed to the individual CDs species. | es_ES |
dc.description.sponsorship | This project has received funding from the European Union’s Horizon 2020 research and innovation programme under the Marie Sklodowska-Curie grant agreement No 642742 | es_ES |
dc.language.iso | eng | es_ES |
dc.publisher | Wiley-VCH | es_ES |
dc.relation | info:eu-repo/grantAgreement/EC/H2020/642742 | es_ES |
dc.relation.isversionof | Postprint | es_ES |
dc.rights | openAccess | en_EN |
dc.subject | Layered transition metal dichalcogenides | es_ES |
dc.subject | Carbon dots | es_ES |
dc.subject | Electrostatic interactions | es_ES |
dc.title | Electronic interactions in illuminated carbon dots/MoS2 ensembles and electrocatalytic activity towards hydrogen evolution | es_ES |
dc.type | artículo | es_ES |
dc.identifier.doi | 10.1002/chem.201801425 | - |
dc.description.peerreviewed | Peer reviewed | es_ES |
dc.relation.publisherversion | https://doi.org/10.1002/chem.201801425 | es_ES |
dc.embargo.terms | 2019-05-15 | es_ES |
dc.contributor.funder | European Commission | es_ES |
dc.relation.csic | Sí | es_ES |
oprm.item.hasRevision | no ko 0 false | * |
dc.identifier.funder | http://dx.doi.org/10.13039/501100000780 | es_ES |
dc.type.coar | http://purl.org/coar/resource_type/c_6501 | es_ES |
item.cerifentitytype | Publications | - |
item.openairecristype | http://purl.org/coar/resource_type/c_18cf | - |
item.grantfulltext | open | - |
item.openairetype | artículo | - |
item.fulltext | With Fulltext | - |
item.languageiso639-1 | en | - |
Aparece en las colecciones: | (ICB) Artículos (ISQCH) Artículos |
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Postprint Chem Eur. J.-2018.pdf | 2,72 MB | Adobe PDF | Visualizar/Abrir | |
Submitted Manuscript.pdf | 768,9 kB | Adobe PDF | Visualizar/Abrir |
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