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dc.contributor.authorPellicer, Eva-
dc.contributor.authorLópez-Ortega, Alberto-
dc.contributor.authorEstrader, Marta-
dc.contributor.authorEstradé, Sònia-
dc.contributor.authorPeiró, Francesca-
dc.contributor.authorGolosovsky, Igor V.-
dc.contributor.authorSuriñach, S.-
dc.contributor.authorBaró, María Dolors-
dc.contributor.authorSort, Jordi-
dc.contributor.authorNogués, Josep-
dc.date.accessioned2014-07-01T10:11:38Z-
dc.date.available2014-07-01T10:11:38Z-
dc.date.issued2013-
dc.identifierdoi: 10.1039/C3NR00989K-
dc.identifierissn: 2040-3364-
dc.identifiere-issn: 2040-3372-
dc.identifier.citationNanoscale 5(12): 5561-5567 (2013)-
dc.identifier.urihttp://hdl.handle.net/10261/99221-
dc.descriptionet al.-
dc.description.abstractThe controlled filling of the pores of highly ordered mesoporous antiferromagnetic Co3O4 replicas with ferrimagnetic FexCo3-xO4 nanolayers is presented as a proof-of-concept toward the integration of nanosized units in highly ordered, heterostructured 3D architectures. Antiferromagnetic (AFM) Co3O 4 mesostructures are obtained as negative replicas of KIT-6 silica templates, which are subsequently coated with ferrimagnetic (FiM) Fe xCo3-xO4 nanolayers. The tuneable magnetic properties, with a large exchange bias and coercivity, arising from the FiM/AFM interface coupling, confirm the microstructure of this novel two-phase core-shell mesoporous material. The present work demonstrates that ordered functional mesoporous 3D-materials can be successfully infiltrated with other compounds exhibiting additional functionalities yielding highly tuneable, versatile, non-siliceous based nanocomposites. © 2013 The Royal Society of Chemistry.-
dc.description.sponsorshipThis work is supported by the 2009-SGR-1292 andCTP2009-00018 projects of the Generalitat de Catalunya, the MAT2010-20616-C02, MAT2011-27380-C02-01, MAT2011-16407 and CSD2009-0013 projects of the Spanish Ministry of Economy and Competitiveness (MINECO) and the ONDA (no. FP7-PEOPLE-2009-IRSES- 247518) and ESTEEM2 (312483, Integrated Infraestructure Initiative-I3, FP7) projects of the European Union. I.V.G. thanks the Generalitat de Catalunya for his sabbatical fellowship (2010 PIV 00096) and the Russian grants RFBR-13-02-00121 and MESRF- 16.518.11.7034. M.E. acknowledges the Spanish Ministry of Science and Innovation through the Juan de la Cierva Program. M.D.B. was partially supported by an ICREA Academia award.-
dc.publisherRoyal Society of Chemistry (UK)-
dc.relationinfo:eu-repo/grantAgreement/EC/FP7/247518-
dc.relationinfo:eu-repo/grantAgreement/EC/FP7/312483-
dc.relation.isversionofPostprint-
dc.rightsclosedAccess-
dc.titleControlled 3D-coating of the pores of highly ordered mesoporous antiferromagnetic Co3O4 replicas with ferrimagnetic FexCo3-xO4 nanolayers-
dc.typeartículo-
dc.identifier.doi10.1039/C3NR00989K-
dc.relation.publisherversionhttp://dx.doi.org/10.1039/C3NR00989K-
dc.date.updated2014-07-01T10:11:38Z-
dc.description.versionPeer Reviewed-
dc.language.rfc3066eng-
dc.contributor.funderMinisterio de Economía y Competitividad (España)-
dc.contributor.funderMinisterio de Ciencia e Innovación (España)-
dc.contributor.funderGeneralitat de Catalunya-
dc.contributor.funderEuropean Commission-
dc.contributor.funderInstitución Catalana de Investigación y Estudios Avanzados-
dc.identifier.funderhttp://dx.doi.org/10.13039/501100003329es_ES
dc.identifier.funderhttp://dx.doi.org/10.13039/501100004837es_ES
dc.identifier.funderhttp://dx.doi.org/10.13039/501100002809es_ES
dc.identifier.funderhttp://dx.doi.org/10.13039/501100000780es_ES
dc.identifier.funderhttp://dx.doi.org/10.13039/501100003741es_ES
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