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Título

Influence of packing on the vibrational properties of infinite and finite bundles of carbon nanotubes

Autor Henrard, Luc; Popov, Valentin N.; Rubio, Angel
Fecha de publicación oct-2001
EditorAmerican Physical Society
Citación Physical Review B 64: 205403 (2001)
ResumenThe quantitative analysis of the vibrational properties of carbon nanotubes is a key issue for the interpretation of Raman experiments. In particular, a reliable characterization of the atomic structure of single-wall carbon nanotubes produced under various conditions is mainly based on the interpretation of low-frequency (100–300 cm-1) Raman spectra. In the present work, we analyze the influence of the packing of the tubes on these low-frequency modes. We find that the low-frequency spectra of crystals of single-wall carbon nanotubes present two intense Raman modes instead of a single fully symmetric A1g mode characteristic of isolated tubes. The second mode has a non-negligible intensity for crystals formed with nanotubes of radii larger than 7 Å. For finite number of tubes in a bundle, two breathinglike intense modes appear as a specific signature. Finally, our simulation for inhomogenous bundles made of a large number of tubes does not reveal any specific signature of the individual tubes in the low-frequency Raman spectra.
Versión del editorhttp://dx.doi.org/10.1103/PhysRevB.64.205403
URI http://hdl.handle.net/10261/98700
DOI10.1103/PhysRevB.64.205403
ISSN1098-0121
E-ISSN1550-235X
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