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Photocatalytic ethanol oxidative dehydrogenation over Pt/TiO 2: Effect of the addition of blue phosphors

AuthorsMurcia, J.J.; Hidalgo, M.C. ; Navío, José Antonio ; Vaiano, V.; Ciambelli, P.; Sannino, D.
Issue Date2012
PublisherHindawi Publishing Corporation
CitationInternational Journal of Photoenergy 2012 (2012)
AbstractEthanol oxidative dehydrogenation over Pt/TiO 2 photocatalyst, in the presence and absence of blue phosphors, was performed. The catalyst was prepared by photodeposition of Pt on sulphated TiO 2. This material was tested in a gas-solid photocatalytic fluidized bed reactor at high illumination efficiency. The effect of the addition of blue phosphors into the fluidized bed has been evaluated. The synthesized catalysts were extensively characterized by different techniques. Pt/TiO 2 with a loading of 0.5wt of Pt appeared to be an active photocatalyst in the selective partial oxidation of ethanol to acetaldehyde improving its activity and selectivity compared to pure TiO 2. In the same way, a notable enhancement of ethanol conversion in the presence of the blue phosphors has been obtained. The blue phosphors produced an increase in the level of ethanol conversion over the Pt/TiO 2 catalyst, keeping at the same time the high selectivity to acetaldehyde. Copyright © 2012 J. J. Murcia et al.
Identifiersdoi: 10.1155/2012/687262
issn: 1110-662X
Appears in Collections:(ICMS) Artículos
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