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Title

Colored and transparent oxide thin films prepared by magnetron sputtering: The glass blower approach

AuthorsGil-Rostra, J. ; Chaboy, Jesús; Yubero, Francisco ; Vilajoana, Antoni; González-Elipe, Agustín R.
Issue Date2013
CitationACS Applied Materials and Interfaces 5(6): 1967-1976 (2013)
AbstractThis work describes the reactive magnetron sputtering processing at room temperature of several mixed oxide MxSiyOz thin films (M: Fe, Ni, Co, Mo, W, Cu) intended for optical, coloring, and aesthetic applications. Specific colors can be selected by adjusting the plasma gas composition and the Si-M ratio in the magnetron target. The microstructure and chemistry of the films are characterized by a large variety of techniques including X-ray photoemission spectroscopy, X-ray absorption spectroscopy (XAS), and infrared spectroscopy, while their optical properties are characterized by UV-vis transmission and reflection analysis. Particularly, XAS analysis of the M cations in the amorphous thin films has provided valuable information about their chemical state and local structure. It is concluded that the M cations are randomly distributed within the SiO2 matrix and that both the M concentration and its chemical state are the key parameters to control the final color of the films. © 2013 American Chemical Society.
URIhttp://hdl.handle.net/10261/96074
DOI10.1021/am302778h
Identifiersdoi: 10.1021/am302778h
issn: 1944-8244
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