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A dense metal-organic framework for enhanced magnetic refrigeration

AuthorsLorusso, Giulia; Palacios, Elias; Roubeau, Olivier; Brechin, Euan K.; Sessoli, Roberta; Evangelisti, Marco
KeywordsGadolinium formate
Magnetocaloric effect
Issue DateSep-2013
CitationAdvanced Materials 25(33): 4653-4656 (2013)
AbstractThe three-dimensional metal-organic framework Gd(HCOO)3 is characterized by a relatively compact crystal lattice of weakly interacting Gd(3+) spin centers interconnected via lightweight formate ligands, overall providing a remarkably large magnetic:non-magnetic elemental weight ratio. The resulting magnetocaloric effect per unit volume is decidedly superior in Gd(HCOO)3 than in the best known magnetic refrigerant materials for liquid-helium temperatures and low-moderate applied fields.
Descriptionet al.
Publisher version (URL)http://dx.doi.org/10.1002/adma.201301997
Appears in Collections:(ICMA) Artículos
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