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Strong enhancement of the lifetime of a resonance state by using a combination of two laser pulses

AuthorsGarcía Vela, Alberto
Issue Date2012
PublisherAmerican Chemical Society
CitationJournal of Physical Chemistry Letters 3: 1941- 1945 (2012)
AbstractThe lifetime of a resonance state overlapping with a second resonance is shown to be strongly enhanced (by a factor of 3) by combining two pump pulses to simultaneously excite the two resonances. Such an enhancement is produced by interference effects occurring between the two coherently excited overlapping resonances. A high degree of control on the intensity of interference, and thus on the resonance lifetime enhancement, is found to be achieved by varying the delay time between the pulses and their relative intensities.
Identifiersdoi: 10.1021/jz300707g
issn: 1948-7185
Appears in Collections:(CFMAC-IFF) Artículos
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