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http://hdl.handle.net/10261/52234
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dc.contributor.author | Yukawa, Yasuhiko | - |
dc.contributor.author | Teat, Simon J. | - |
dc.contributor.author | Roubeau, Olivier | - |
dc.contributor.author | Evangelisti, Marco | - |
dc.contributor.author | Cremades, Eduard | - |
dc.contributor.author | Ruiz, Eliseo | - |
dc.contributor.author | Barrios, L. A. | - |
dc.contributor.author | Aromí, Guillem | - |
dc.date.accessioned | 2012-06-26T10:18:40Z | - |
dc.date.available | 2012-06-26T10:18:40Z | - |
dc.date.issued | 2011 | - |
dc.identifier | doi: 10.1002/chem.201100769 | - |
dc.identifier | issn: 0947-6539 | - |
dc.identifier | e-issn: 1521-3765 | - |
dc.identifier.citation | Chemistry - A European Journal 17(30): 8264-8268 (2011) | - |
dc.identifier.uri | http://hdl.handle.net/10261/52234 | - |
dc.description.abstract | Water is the glue in bridging two [GdNi3] heterometallic fragments to form the new molecular cluster [Et4N][Gd 2Ni6(val)12(MeCN)6(H 2O)3][Gd(NO3)5](ClO 4)5 (1, val= valine anion, see figure), otherwise cemented by amino acid ligands. The shape of the complex cation of 1 resembles an ancient goblet, and its structure holds weak magnetic exchange pathways, as confirmed theoretically and experimentally; this confers the cluster ideal conditions to exhibit good magnetocaloric properties. | - |
dc.description.sponsorship | The authors thank the Generalitat de Catalunya for the prize ICREA Academia 2008 (G.A.) and Grant 2009SGR-1459 (E.C. and E.R.) and Spanish MCI through CTQ2009–06959 (G.A., L.B.), MAT2009-13977- C03 (M.E.), and CTQ2008–06670-C02–01 (E.C., ER). The advanced light source (S.J.T.) is supported by the U.S. Department of Energy (DE-AC02–05CH11231). | - |
dc.language.iso | eng | - |
dc.publisher | Wiley-VCH | - |
dc.rights | closedAccess | - |
dc.title | A molecular pair of [GdNi3] tetrahedra bridged by water molecules | - |
dc.type | artículo | - |
dc.identifier.doi | 10.1002/chem.201100769 | - |
dc.relation.publisherversion | http://dx.doi.org/10.1002/chem.201100769 | - |
dc.date.updated | 2012-06-26T10:18:41Z | - |
dc.description.version | Peer Reviewed | - |
dc.contributor.funder | Generalitat de Catalunya | - |
dc.contributor.funder | Ministerio de Ciencia e Innovación (España) | - |
dc.contributor.funder | Department of Energy (US) | - |
dc.identifier.funder | http://dx.doi.org/10.13039/501100002809 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100004837 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/100000015 | es_ES |
dc.type.coar | http://purl.org/coar/resource_type/c_6501 | es_ES |
item.openairetype | artículo | - |
item.cerifentitytype | Publications | - |
item.languageiso639-1 | en | - |
item.grantfulltext | none | - |
item.openairecristype | http://purl.org/coar/resource_type/c_18cf | - |
item.fulltext | No Fulltext | - |
Aparece en las colecciones: | (ICMA) Artículos |
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