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http://hdl.handle.net/10261/47812
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Campo DC | Valor | Lengua/Idioma |
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dc.contributor.author | Luis, Fernando | - |
dc.contributor.author | Martínez Pérez, M. J. | - |
dc.contributor.author | Montero, Oscar | - |
dc.contributor.author | Sesé Monclús, Javier | - |
dc.contributor.author | Drung, D. | - |
dc.contributor.author | Schurig, T. | - |
dc.date.accessioned | 2012-04-02T11:10:31Z | - |
dc.date.available | 2012-04-02T11:10:31Z | - |
dc.date.issued | 2010-08 | - |
dc.identifier.citation | Physical Review B 82(6): 060403(R) (2010) | es_ES |
dc.identifier.issn | 1098-0121 | - |
dc.identifier.uri | http://hdl.handle.net/10261/47812 | - |
dc.description | 4 páginas, 4 figuras.-- PACS number(s): 75.50.Xx, 75.45.+j, 76.30.Kg, 75.40.Gb.-- et al. | es_ES |
dc.description.abstract | We investigate the mechanism of spin-lattice relaxation of Er ions encapsulated in polyoxometalate clusters, which below 4 K can only reverse its spin via quantum tunneling processes. The temperature-independent rate τ−1 is, at zero field, ten orders of magnitude larger than the rates predicted for direct phonon-induced processes. In addition, we observe that τ−1 is suppressed by external magnetic bias and hyperfine interactions but enhanced by increasing the concentration of Er ions. The observed relaxation agrees with predictions for pure quantum tunneling, showing that this phenomenon drives the thermalization of electronic spins. A possible link between these two phenomena is discussed, involving the collective emission of phonons from particular spin configurations attained via quantum tunneling. | es_ES |
dc.description.sponsorship | The present work has been partly funded by grant MOLSpinQIP from the EU, grants Molecular Nanoscience (Consolider Ingenio 2010 Program), MOLCHIP, M3EM and NANOMOL from the Spanish MICINN, grant NABISUP from DGA, and the PROMETEO Program from the Generalidad Valenciana. | es_ES |
dc.language.iso | eng | es_ES |
dc.publisher | American Physical Society | es_ES |
dc.rights | openAccess | es_ES |
dc.title | Spin-lattice relaxation via quantum tunneling in an Er3+-polyoxometalate molecular magnet | es_ES |
dc.type | artículo | es_ES |
dc.identifier.doi | 10.1103/PhysRevB.82.060403 | - |
dc.description.peerreviewed | Peer reviewed | es_ES |
dc.relation.publisherversion | http://dx.doi.org/10.1103/PhysRevB.82.060403 | es_ES |
dc.identifier.e-issn | 1550-235X | - |
dc.type.coar | http://purl.org/coar/resource_type/c_6501 | es_ES |
item.languageiso639-1 | en | - |
item.fulltext | With Fulltext | - |
item.openairecristype | http://purl.org/coar/resource_type/c_18cf | - |
item.cerifentitytype | Publications | - |
item.grantfulltext | open | - |
item.openairetype | artículo | - |
Aparece en las colecciones: | (ICMA) Artículos |
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Spin-lattice relaxation.pdf | 820,47 kB | Adobe PDF | Visualizar/Abrir |
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