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Title

Synthesis and Characterization of Carbon-Based Heterogeneous Catalysts for Energy Release of Molecular Solar Thermal Energy Storage Materials

AuthorsMagson, Lucien; Hölzel, Helen; Aslam, Adil S.; Henninger, Stefan; Munz, Gunther; Moth-Poulsen, Kasper; Knaebbeler-Buss, Markus; Funes Ardoiz, Ignacio; Sampedro, Diego
KeywordsMOST systems
Abundant metals
Energy storage
Heterogeneous catalysts
Isomerization
Issue Date14-Feb-2024
PublisherAmerican Chemical Society
CitationACS Applied Materials and Interfaces 16(6): 7211–7218 (2024)
AbstractMolecular solar thermal energy storage (MOST) systems are rapidly becoming a feasible alternative to energy storage and net-zero carbon emission heating. MOST systems involve a single photoisomerization pair that incorporates light absorption, storage, and heat release processes in one recurring cycle. Despite significant recent advancements in the field, the catalytic back-reaction from MOST systems remains relatively unexplored. A wide range of applications is possible, contingent on the energy densities of the specific photoisomers. Here, we report platinum-, copper-, and nickel-based heterogeneous catalysts screened in batch conditions for the back-conversion reaction on the cyano-3-(4-methoxyphenyl)-norbornadiene/quadricyclane pair. Catalyst reactivities are investigated using structural characterization, imaging techniques, and spectroscopic analysis. Finally, the thermal stability is also explored for our best-performing catalysts.
Publisher version (URL)http://doi.org/10.1021/acsami.3c16855
URIhttp://hdl.handle.net/10261/347482
DOI10.1021/acsami.3c16855
ISSN1944-8244
Appears in Collections:(ICMAB) Artículos




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