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Title

Low-Voltage, Dual-Gate Organic Transistors with High Sensitivity and Stability toward Electrostatic Biosensing

AuthorsNikolka, Mark; Simatos, Dimitrios; Foudeh, Amir; Pfattner, Raphael CSIC ORCID ; McCulloch, Iain; Bao, Zhenan
KeywordsOrganic electronics
Polymer devices
Field-effect transistors
Low voltage
Bioelectronics
Sensing
Ionic dielectric
Issue Date9-Sep-2020
PublisherAmerican Chemical Society
CitationACS Applied Materials and Interfaces 12(36): 40581-40589 (2020)
AbstractHigh levels of performance and stability have been demonstrated for conjugated polymer thin-film transistors in recent years, making them promising materials for flexible electronic circuits and displays. For sensing applications, however, most research efforts have been focusing on electrochemical sensing devices. Here we demonstrate a highly stable biosensing platform using polymer transistors based on the dual-gate mechanism. In this architecture a sensing signal is transduced and amplified by the capacitive coupling between a low-k bottom dielectric and a high-k ionic elastomer top dielectric that is in contact with an analyte solution. The new design exhibits a high signal amplification, high stability under bias stress in various aqueous environments, and low signal drift. Our platform, furthermore, while responding expectedly to charged analytes such as the protein bovine serum albumin, is insensitive to changes of salt concentration of the analyte solution. These features make this platform a potentially suitable tool for a variety of biosensing applications.
Publisher version (URL)http://dx.doi.org/10.1021/acsami.0c10201
URIhttp://hdl.handle.net/10261/234325
ISSN1944-8244
Appears in Collections:(ICMAB) Artículos
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