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Title

Bimetallic PdAu catalysts for formic acid dehydrogenation

AuthorsSantos, Jose Luis; Leon, Claudia; Monnier, G.; Ivanova, Svetlana ; Centeno, Miguel Ángel ; Odriozola, José Antonio
KeywordsFormic Acid dehydrogenation
Hydrogen economy
Palladium
Gold
bimetallic catalyst.
Issue Date2020
PublisherPergamon Press
CitationInternational Journal of Hydrogen Energy (2020)
AbstractA series of monometallic and bimetallic palladium gold catalyst were prepared and studied for the formic acid dehydrogenation reaction. Different Pd/Au compositions were employed (PdAu, where x = 25; 50 and 75) and their impact on alloy structure, particle size and dispersion was evaluated. Active phase composition and reaction parameters such as temperature, formic acid concentration or formate/formic acid ratio were adjusted to obtain active and selective catalyst for hydrogen production. An important particle size effect was observed and related to Pd/Au composition for all bimetallic catalysts.
Publisher version (URL)http://dx.doi.org/10.1016/j.ijhydene.2020.06.076
URIhttp://hdl.handle.net/10261/219640
DOIhttp://dx.doi.org/10.1016/j.ijhydene.2020.06.076
Identifiersdoi: 10.1016/j.ijhydene.2020.06.076
issn: 0360-3199
Appears in Collections:(ICMS) Artículos
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