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dc.contributor.authorCastillo-Blas, Ceciliaes_ES
dc.contributor.authorÁlvarez-Galván, Consueloes_ES
dc.contributor.authorPuente-Orench, Inéses_ES
dc.contributor.authorGarcía-Sánchez, Albaes_ES
dc.contributor.authorOropeza, Freddy E.es_ES
dc.contributor.authorGutiérrez-Puebla, Enriquees_ES
dc.contributor.authorMonge, M. Ángeleses_ES
dc.contributor.authorPeña O'Shea, Víctor A. de laes_ES
dc.contributor.authorGándara Barragán, Felipees_ES
dc.date.accessioned2020-09-01T12:09:05Z-
dc.date.available2020-09-01T12:09:05Z-
dc.date.issued2020-
dc.identifier.citationNano Research: (2020)es_ES
dc.identifier.issn1998-0124-
dc.identifier.urihttp://hdl.handle.net/10261/218949-
dc.description.abstractThe precise control on the combination of multiple metal atoms in the structure of metal-organic frameworks (MOFs) endowed by reticular chemistry, allows the obtaining of materials with compositions that are programmed for achieving enhanced reactivity. The present work illustrates how through the transformation of MOFs with desired arrangements of metal cations, multi-metal spinel oxides with precise compositions can be obtained, and used as catalyst precursor for the reverse water-gas shift reaction. The differences in the spinel initial composition and structure, determined by neutron powder diffraction, influence the overall catalytic activity with changes in the process of in situ formation of active, metal-oxide supported metal nanoparticles, which have been monitored and characterized with in situ X-ray diffraction and photoelectron spectroscopy studies.es_ES
dc.description.sponsorshipWork at Instituto de Ciencia de Materiales de Madrid–Consejo Superior de Instigaciones Científicas (CSIC) has been supported by the Spanish Research Agency (Agencia Estatal de Investigación, AEI), Projects MAT2016-78465-R and CTQ2017-87262-R. This work was supported by the EU (ERC CoG HyMAP 648319) and Spanish MINECO (ENE2016-79608-C2-1-R). Authors also wish to thank to “Comunidad de Madrid” and European Structural Funds for their financial support to FotoArt-CM project (S2018/NMT-4367). F. G. acknowledges financial support from MINECO Ramón y Cajal program (RyC-2015-18384).es_ES
dc.language.isoenges_ES
dc.publisherSpringer Naturees_ES
dc.relationS2018/NMT-4367/FotoArt-CMes_ES
dc.relationMINECO/ICTI2013-2016/MAT2016-78465-Res_ES
dc.relationMICIU/ICTI2017-2020/CTQ2017-87262-Res_ES
dc.relationMINECO/ICTI2013-2016CTQ2017-87262-RVes_ES
dc.relationinfo:eu-repo/grantAgreement/EC/H2020/648319es_ES
dc.relationMINECO/ICTI2013-2016/ENE2016-79608-C2-1-Res_ES
dc.relationMINECO/ICTI2013-2016/RYC-2015-18384es_ES
dc.rightsclosedAccesses_ES
dc.titleHighly efficient multi-metal catalysts for carbon dioxide reduction prepared from atomically sequenced metal organic frameworkses_ES
dc.typeartículoes_ES
dc.identifier.doi10.1007/s12274-020-2813-x-
dc.description.peerreviewedPeer reviewedes_ES
dc.relation.publisherversionhttps://doi.org/10.1007/s12274-020-2813-xes_ES
dc.identifier.e-issn1998-0000-
dc.contributor.funderMinisterio de Economía y Competitividad (España)es_ES
dc.contributor.funderAgencia Estatal de Investigación (España)es_ES
dc.contributor.funderMinisterio de Ciencia, Innovación y Universidades (España)es_ES
dc.contributor.funderEuropean Commissiones_ES
dc.contributor.funderEuropean Research Counciles_ES
dc.contributor.funderComunidad de Madrides_ES
dc.relation.csices_ES
oprm.item.hasRevisionno ko 0 false*
dc.identifier.funderhttp://dx.doi.org/10.13039/501100000780es_ES
dc.identifier.funderhttp://dx.doi.org/10.13039/501100003329es_ES
dc.identifier.funderhttp://dx.doi.org/10.13039/501100000781es_ES
dc.identifier.funderhttp://dx.doi.org/10.13039/100012818es_ES
dc.identifier.funderhttp://dx.doi.org/10.13039/501100011033es_ES
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