English   español  
Please use this identifier to cite or link to this item: http://hdl.handle.net/10261/218949
Share/Impact:
Statistics
logo share SHARE logo core CORE   Add this article to your Mendeley library MendeleyBASE

Visualizar otros formatos: MARC | Dublin Core | RDF | ORE | MODS | METS | DIDL
Exportar a otros formatos:

Title

Highly efficient multi-metal catalysts for carbon dioxide reduction prepared from atomically sequenced metal organic frameworks

AuthorsCastillo-Blas, Cecilia; Álvarez-Galván, Consuelo; Puente-Orench, Inés; García-Sánchez, Alba; Oropeza, Freddy E.; Gutiérrez-Puebla, Enrique ; Monge, M. Ángeles ; Peña O'Shea, Víctor A. de la; Gándara Barragán, Felipe
Issue Date2020
PublisherSpringer Nature
CitationNano Research: (2020)
AbstractThe precise control on the combination of multiple metal atoms in the structure of metal-organic frameworks (MOFs) endowed by reticular chemistry, allows the obtaining of materials with compositions that are programmed for achieving enhanced reactivity. The present work illustrates how through the transformation of MOFs with desired arrangements of metal cations, multi-metal spinel oxides with precise compositions can be obtained, and used as catalyst precursor for the reverse water-gas shift reaction. The differences in the spinel initial composition and structure, determined by neutron powder diffraction, influence the overall catalytic activity with changes in the process of in situ formation of active, metal-oxide supported metal nanoparticles, which have been monitored and characterized with in situ X-ray diffraction and photoelectron spectroscopy studies.
Publisher version (URL)https://doi.org/10.1007/s12274-020-2813-x
URIhttp://hdl.handle.net/10261/218949
DOI10.1007/s12274-020-2813-x
ISSN1998-0124
E-ISSN1998-0000
Appears in Collections:(ICP) Artículos
(ICMM) Artículos
(ICMA) Artículos
Files in This Item:
File Description SizeFormat 
accesoRestringido.pdf59,24 kBAdobe PDFThumbnail
View/Open
Show full item record
Review this work
 


WARNING: Items in Digital.CSIC are protected by copyright, with all rights reserved, unless otherwise indicated.