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Natural Deep Eutectic Solvents as Performance Additivesfor Peroxygenase Catalysis

AuthorsMa, Yanhang; Li, Yongru; Ali, Shahid; Li, Peilin; Zhang, Wuyuan; Rauch, Marine C. R.; Willot, Sébastien J.-P.; Ribitsch, Doris; Choi, Young Hae; Alcalde Galeote, Miguel ; Hollmann, Frank; Wang, Yonghua
Deep Eutectic Solvents
Oxyfunctionalisation reactions
Issue Date17-Dec-2020
PublisherChemPubSoc Europe
CitationChemCatChem 2020, 12, 989–994
Abstract[EN] Natural deep eutectic solvents (NADES) are proposed as alternative solvents for peroxygenase-catalysed oxyfunctionali-zation reactions. Choline chloride-based NADES are of particularinterest as they can serve as solvent, enzyme-stabiliser and sacrificial electron donor for the in situ H2O2generation. This report provides the first proof-of-concept and basic character-isation of this new reaction system. Highly promising turnovernumbers for the biocatalysts of up to 200,000 have been achieved.
Publisher version (URL)http://dx.doi.org/10.1002/cctc.201901842
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