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Title

Expanding the Spectrum of Light-Driven Peroxygenase Reactions

AuthorsWillot, S.J.P.; Fernández-Fueyo, Elena ; Tieves, Florian; Pesic, Milja; Alcalde Galeote, Miguel ; Arends, W.C.E. Isabel; Park, Chan Beum; Hollmann, Frank
KeywordsBiocatalysis
Formate dehydrogenase
Hydrogen peroxide formation
Oxyfunctionalization
Peroxygenases
Photocatalysis
Issue Date2019
PublisherAmerican Chemical Society
CitationACS Catalysis 9: 890- 894 (2019)
Abstract[EN] Peroxygenases require a controlled supply of HO to operate efficiently. Here, we propose a photocatalytic system for the reductive activation of ambient O to produce HO which uses the energy provided by visible light more efficiently based on the combination of wavelength-complementary photosensitizers. This approach was coupled to an enzymatic system to make formate available as a sacrificial electron donor. The scope and current limitations of this approach are reported and discussed.
Publisher version (URL)http://dx.doi.org/10.1021/acscatal.8b03752
URIhttp://hdl.handle.net/10261/214960
Identifiersdoi: 10.1021/acscatal.8b03752
e-issn: 2155-5435
Appears in Collections:(ICP) Artículos
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