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| Title: | A New Mechanism of Acid Rain Generation from HOSO at the Air-Water Interface |
| Authors: | Ruiz-López, M.F.; Martins-Costa, M.T.C.; Anglada Rull, Josep M.  ; Francisco, J.S. |
| Issue Date: | 2019 |
| Publisher: | American Chemical Society |
| Citation: | Journal of the American Chemical Society 141: 16564- 16568 (2019) |
| Abstract: | The photochemistry of SO at the air-water interface of water droplets leads to the formation of HOSO radicals. Using first-principles simulations, we show that HOSO displays an unforeseen strong acidity (pK = -1) comparable with that of nitric acid and is fully dissociated at the air-water interface. Accordingly, this radical might play an important role in acid rain formation. Potential implications are discussed. |
| Publisher version (URL): | http://dx.doi.org/10.1021/jacs.9b07912 |
| URI: | http://hdl.handle.net/10261/210513 |
| Identifiers: | doi: 10.1021/jacs.9b07912 issn: 1520-5126 |
| Appears in Collections: | (IQAC) Artículos |
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| File | Description | Size | Format | |
|---|---|---|---|---|
| A New Mechanism of Acid Rain Generation from HOSO at the Air-Water Interface.pdf Embargoed until October 7, 2020 | 3,16 MB | Adobe PDF |  View/Open Request a copy |
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