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A New Mechanism of Acid Rain Generation from HOSO at the Air-Water Interface

AuthorsRuiz-López, M.F.; Martins-Costa, M.T.C.; Anglada Rull, Josep M. ; Francisco, J.S.
Issue Date2019
PublisherAmerican Chemical Society
CitationJournal of the American Chemical Society 141: 16564- 16568 (2019)
AbstractThe photochemistry of SO at the air-water interface of water droplets leads to the formation of HOSO radicals. Using first-principles simulations, we show that HOSO displays an unforeseen strong acidity (pK = -1) comparable with that of nitric acid and is fully dissociated at the air-water interface. Accordingly, this radical might play an important role in acid rain formation. Potential implications are discussed.
Publisher version (URL)http://dx.doi.org/10.1021/jacs.9b07912
Identifiersdoi: 10.1021/jacs.9b07912
issn: 1520-5126
Appears in Collections:(IQAC) Artículos
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