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http://hdl.handle.net/10261/198390
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dc.contributor.author | Arancibia Miranda, Nicolás | - |
dc.contributor.author | Escudey, Mauricio | - |
dc.contributor.author | Pizarro, C. | - |
dc.contributor.author | Denardin, Juliano C. | - |
dc.contributor.author | García-González, M. T. | - |
dc.contributor.author | Fabris, J. D. | - |
dc.contributor.author | Charlet, Laurent | - |
dc.date.accessioned | 2020-01-20T16:16:47Z | - |
dc.date.available | 2020-01-20T16:16:47Z | - |
dc.date.issued | 2014-03 | - |
dc.identifier | doi: 10.1016/j.materresbull.2013.12.014 | - |
dc.identifier | issn: 0025-5408 | - |
dc.identifier.citation | Materials Research Bulletin 51: 145-152 (2014) | - |
dc.identifier.uri | http://hdl.handle.net/10261/198390 | - |
dc.description.abstract | A chemical method to synthesize a magnetite coating on aluminosilicate nanotubes (imogolite) that can be used as a magnetic adsorptive composite is reported via a new procedure based on impregnation with excess of solvent. This produced a nanocomposite of imogolite and magnetite, retaining at least two of the individual properties of its initial chemical species, which are determinant for some technological applications: large surface area and high saturation magnetization. Comparatively significant differences in terms of electrophoretic and magnetic characteristics were found between the direct solid mixture of the starting materials and the resultant imogolite-magnetite mixture. The adsorption kinetics of arsenate is described adequately by the pseudo-second model and the maximum adsorbed amounts (qe) of this anion were closed to those obtained experimentally. A high rate of arsenate adsorption on Fe-imogolite was initially observed, suggesting that the formation of new surface sites qualitatively and quantitatively improve the removal of arsenate. The combined use of different characterization techniques (XRD, TEM, Mössbauer spectroscopy, EM, VSM and SQUID) and the kinetic sorption study suggest that Fe-imogolite has a large potential for the treatment of arsenate polluted water or other nanotechnological applications, due to its high chemical reactivity. © 2013 Elsevier Ltd. | - |
dc.description.sponsorship | This work was supported by FONDECYT under Project 1070116; by Proyecto de Inserción en la Academia 79090022; Center for the Development of Nanoscience and Nanotechnology (CEDENNA); by the Spanish Ministry of Science and Innovation (AGL 2005-07017-C03-03); and by the Brazilian agencies CNPq (grants 302479/2010-4 and Prosul 490096/2010-7) and FAPEMIG (PPM 00419-10). We are especially grateful to Mr. F. Pinto, Mr. M. Juanco and Dr. Martín Treps for their technical assistance. N. Arancibia-Miranda acknowledges a scholarship from CONICYT (Chile) and CAPES (Brazil) for granting the Visiting Professor PVNS fellowship to JDF at UFVJM. | - |
dc.language | eng | - |
dc.publisher | Elsevier BV | - |
dc.rights | closedAccess | - |
dc.subject | A. Amorphous materials | - |
dc.subject | A. Magnetic materials | - |
dc.subject | C. Mössbauer spectroscopy | - |
dc.subject | D. Magnetic properties | - |
dc.subject | D. Surface properties | - |
dc.title | Preparation and characterization of a single-walled aluminosilicate nanotube-iron oxide composite: Its applications to removal of aqueous arsenate | - |
dc.type | artículo | - |
dc.identifier.doi | 10.1016/j.materresbull.2013.12.014 | - |
dc.relation.publisherversion | http://dx.doi.org/10.1016/j.materresbull.2013.12.014 | - |
dc.date.updated | 2020-01-20T16:16:47Z | - |
dc.contributor.funder | Fondo Nacional de Desarrollo Científico y Tecnológico (Chile) | - |
dc.contributor.funder | Centro para el Desarrollo de la Nanociencia y la Nanotecnología (Chile) | - |
dc.contributor.funder | Ministerio de Ciencia e Innovación (España) | - |
dc.contributor.funder | Conselho Nacional de Desenvolvimento Científico e Tecnológico (Brasil) | - |
dc.contributor.funder | Fundação de Amparo à Pesquisa do Estado de São Paulo Minas Gerais | - |
dc.contributor.funder | Comisión Nacional de Investigación Científica y Tecnológica (Chile) | - |
dc.contributor.funder | Coordenação de Aperfeiçoamento de Pessoal de Nível Superior (Brasil) | - |
dc.relation.csic | Sí | - |
dc.identifier.funder | http://dx.doi.org/10.13039/501100004837 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100003593 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100004901 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100002322 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100002848 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100002850 | es_ES |
dc.type.coar | http://purl.org/coar/resource_type/c_6501 | es_ES |
item.openairetype | artículo | - |
item.grantfulltext | none | - |
item.cerifentitytype | Publications | - |
item.openairecristype | http://purl.org/coar/resource_type/c_18cf | - |
item.fulltext | No Fulltext | - |
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