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Título: | Possible Bose-Einstein condensate associated with an orbital degree of freedom in the Mott insulator CaCr O3 |
Autor: | Zhou, J. S.; Cao, L. P.; Alonso, J. A. CSIC ORCID; Sanchez-Benitez, J.; Fernández-Díaz, M. T.; Li, X.; Cheng, J. G.; Marshall, L. G.; Jin, C. Q.; Goodenough, J. B. | Fecha de publicación: | 15-oct-2016 | Editor: | American Physical Society | Citación: | Physical Review - Section B - Condensed Matter 94(15): 155137 (2016) | Resumen: | Whether CaCrO3 is a Mott insulator or a correlated metal is still controversial. We have performed measurements of magnetization, specific heat, and thermal conductivity on CaCrO3 samples selected from many batches of high-pressure synthesis. The single-crystal CaCrO3 sample exhibits an unprecedentedly sharp transition at a Néel temperature TN≈90K. The critical behavior of specific heat cannot be rationalized by the renormalization group theory for a second-order magnetic transition. More surprisingly, the thermal conductivity κ exhibits an anomalous drop on cooling through TN, which is opposite to all known influence on κ from either spin or orbital ordering. We have argued, on the basis of anomalies found in all three measurements and structural data, for the coexistence of itinerant π-bonding electrons in a c-axis band and localized xy electrons in xy orbitals responsible for type-C antiferromagnetic order below TN and the occupation of a pure, localized xy orbital undergoing a Bose-Einstein condensate at TN. | Versión del editor: | https://doi.org/10.1103/PhysRevB.94.155137 | URI: | http://hdl.handle.net/10261/186954 | DOI: | 10.1103/PhysRevB.94.155137 | Identificadores: | doi: 10.1103/PhysRevB.94.155137 e-issn: 1550-235X issn: 1098-0121 |
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