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Título

An apparatus for quantitative high-harmonic generation spectroscopy in molecular vapours

AutorMcGrath, Felicity; Johnson, Allan S.; Austin, Dane R.; Hawkins, Peter; Wood, David; Miseikis, Lukas; Simpson, Emma R.; Castillejo, Marta ; Torres, Ricardo; Parker, Susana; Siegel, Thomas; Marangos, Jon P.
Fecha de publicación2017
EditorAmerican Physical Society
CitaciónReview of Scientific Instruments 88(10),103108
ResumenWe present an apparatus for performing gas phase high-harmonic generation spectroscopy of molecules primarily found in the liquid phase. Liquid molecular samples are heated in a temperature controlled bath and their vapour is used to back a continuous ow gas jet, with vapour pressures of over 1 bar possible. In order to demonstrate the system, we perform high harmonic spectroscopy experiments in benzene with a 1.8 µm driving field. Using the unique capabilities of the system, we obtain spectra that are nearly free from the effects of longitudinal phase-matching, amenable to comparison with advanced numerical modelling.
Versión del editorhttp://aip.scitation.org/doi/10.1063/1.4986037
URIhttp://hdl.handle.net/10261/157860
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