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In-Situ Scrutiny of the Relationship between Polymorphic Phases and Properties of Self-Assembled Monolayers of a Biphenyl Based Thiol

AutorParadinas, Markos; Munuera, Carmen; Buck, Manfred; Ocal, Carmen
Fecha de publicación4-ago-2017
EditorAmerican Chemical Society
CitaciónJournal of Physical Chemistry B - Condensed Phase: 10.1021/acs.jpcb.7b05958 (2017)
ResumenTwo polymorphic phases of ω-(4′-methylbiphenyl-4-yl) butane-1-thiol (BP4) molecules formed on Au(111) were investigated by multidimensional atomic force microscopy, combining conductivity measurements, electrostatic characterization, friction force mapping, and normal force spectroscopy. Based on the same molecular structure but differing in molecular order, packing density, and molecular tilt, the two phases serve as a test bench to establish the structure–property relationships in self-assembled monolayers (SAMs). From a detailed analysis of the charge transport and electrostatics, the contributions of geometrical and electronic effects to the tunneling are discussed.
Versión del editorhttp://dx.doi.org/10.1021/acs.jpcb.7b05958
URIhttp://hdl.handle.net/10261/155974
DOI10.1021/acs.jpcb.7b05958
ISSN1520-6106
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