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dc.contributor.authorDörling, Bernhardes_ES
dc.contributor.authorSánchez Díaz, Antonioes_ES
dc.contributor.authorArteaga, Orioles_ES
dc.contributor.authorVeciana, Andreaes_ES
dc.contributor.authorAlonso Carmona, M. Isabeles_ES
dc.contributor.authorCampoy Quiles, Marianoes_ES
dc.date.accessioned2017-09-05T12:36:59Z-
dc.date.available2017-09-05T12:36:59Z-
dc.date.issued2017-07-31-
dc.identifier.citationAdvanced Optical Materials: 10.1002/adom.201700276 (2017)es_ES
dc.identifier.issn2195-1071-
dc.identifier.urihttp://hdl.handle.net/10261/154781-
dc.description.abstractThe nucleation of single macroscopic spherulites at desired positions, as well as ordered arrays of multiple spherulites, is demonstrated by combining the use of crystallizable solvents with local control of solvent evaporation during solution deposition. Moreover, the temperature assisted localized frustration of molecular orientation is shown, enabling the fabrication of samples containing both isotropic areas and spherulites. These macroscopic circular polycrystalline structures are characterized using a range of polarized spectroscopic techniques that allow quantifying their large degree of chain orientation. In order to show the potential of these large conjugated polymer spherulites centered at desired locations, graded bilayer organic photovoltaic devices were fabricated to be used as polarimeters, solid state light polarization detectors with no moving parts, and position sensitive photodetectors.es_ES
dc.description.sponsorshipThe authors would like to acknowledge financial support from the Ministerio de Economía y Competitividad of Spain through the “Severo Ochoa” Programme for Centers of Excellence in R&D (SEV-2015- 0496) and projects CSD2010-00044 (Consolider NANOTHERM) and MAT2015-70850-P; CSIC through project 201560I032; and the European Research Council (ERC) under grant agreement no. 648901. The authors would like to thank Mr. Javier Fernández Tejero and Ms. Laura Córcoles Guija for their contribution toward putting together the LBIC system and Andrés Gomez for the AFM measurements. The authors are grateful to Dr. Miquel Garriga (ICMAB) and Dr. Alejandro Goñi (ICMAB) for useful discussions. The residents of Sant Pol de Mar are sincerely acknowledged for inspiration regarding a sundial that works in the shade.es_ES
dc.language.isoenges_ES
dc.publisherWiley-VCHes_ES
dc.relationMINECO/ICTI2013-2016/SEV-2015-0496es_ES
dc.relationMINECO/ICTI2013-2016/MAT2015-70850-Pes_ES
dc.relationinfo:eu-repo/grantAgreement/EC/H2020/648901es_ES
dc.relation.isversionofPublisher's versiones_ES
dc.rightsopenAccesses_ES
dc.subjectConjugated polymerses_ES
dc.subjectMolecular orientationes_ES
dc.subjectPhotovoltaic deviceses_ES
dc.subjectSensores_ES
dc.subjectPolarizationes_ES
dc.titleControlled Pinning of Conjugated Polymer Spherulites and Its Application in Detectorses_ES
dc.typeartículoes_ES
dc.identifier.doihttp://dx.doi.org/10.1002/adom.201700276-
dc.description.peerreviewedPeer reviewedes_ES
dc.relation.publisherversionhttp://dx.doi.org/10.1002/adom.201700276es_ES
dc.rights.licensehttps://creativecommons.org/licenses/by/4.0/es_ES
dc.contributor.funderMinisterio de Economía y Competitividad (España)es_ES
dc.contributor.funderEuropean Research Counciles_ES
dc.contributor.funderConsejo Superior de Investigaciones Científicas (España)es_ES
dc.relation.csices_ES
oprm.item.hasRevisionno ko 0 false*
dc.identifier.funderhttp://dx.doi.org/10.13039/501100000781es_ES
dc.identifier.funderhttp://dx.doi.org/10.13039/501100003329es_ES
dc.identifier.funderhttp://dx.doi.org/10.13039/501100003339es_ES
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