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Observation of rotationally mediated focused inelastic resonances in D2 scattering from Cu(001)

AutorBertino, M.F.; Miret-Artés, Salvador ; Toennies, J.P.; Benedek, G.
Fecha de publicación15-oct-1997
EditorAmerican Physical Society
CitaciónPhysical Review B 56: 9964- 9969 (1997)
ResumenRotationally mediated focused inelastic resonances (RMFIR's) in the angular distributions of D2 scattered from Cu(001) are observed. The FIR effect involves a phonon-assisted focusing of an incident beam of arbitrary energy and direction into a final channel of one single well-defined energy and direction. Surprisingly for an incident energy Ei = 27 meV the RMFIR conditions for the scattered beam coincide with the kinematic conditions required for a further elastic selective adsorption mechanism called the rotationally mediated critical kinematic (RMCK) effect. By taking advantage of the RMFIR and elastic RMCK effects, three effective bound states of energy ¿n,J = -21.5 meV, -12.4 meV, and -10.3 meV are determined. They are attributed to the lowest bound states ¿0 = -28.9 meV and ¿1 = -19.8 meV combined with the rotational excitation energy for J = 1 to be BrotJ(J + 1) = 7.41 meV, respectively, and ¿3 = -10.3 meV combined with the rotational ground state (J = 0). While the ¿1 and ¿3 states appear as maxima in the angular distribution at RMFIR conditions, the ¿0 yields a striking minimum which represents the first evidence of what we call an anti-FIR feature. Theoretical arguments to explain the different FIR signatures observed are provided. A fit of a phenomenological interaction potential to the experimental bound-state values yields a value for the well depth D = 32.5 meV which is somewhat deeper than that found previously. © 1997 The American Physical Society
Descripción6 págs.; 4 figs.; 1 tab.
Versión del editorhttps://doi.org/10.1103/PhysRevB.56.9964
Identificadoresdoi: 10.1103/PhysRevB.56.9964
issn: 0163-1829
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