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http://hdl.handle.net/10261/137668
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dc.contributor.author | López Periago, Ana M. | - |
dc.contributor.author | Vallcorba, Oriol | - |
dc.contributor.author | Frontera, Carlos | - |
dc.contributor.author | Domingo, Concepción | - |
dc.contributor.author | Ayllón, José A. | - |
dc.date.accessioned | 2016-10-04T10:27:24Z | - |
dc.date.available | 2016-10-04T10:27:24Z | - |
dc.date.issued | 2015-03-09 | - |
dc.identifier | issn: 1477-9234 | - |
dc.identifier.citation | Dalton Transactions 44: 7548-7553 (2015) | - |
dc.identifier.uri | http://hdl.handle.net/10261/137668 | - |
dc.description.abstract | The preparation of copper(II) one-dimensional MOFs using an eco-efficient method is reported here. This method is based exclusively on using supercritical CO<inf>2</inf> as a solvent, without the addition of any other additive or co-solvent. Neutral acetylacetonate copper complexes and two linear linkers, namely, the bidentate 4,4¿-bipyridine and 4,4¿-trimethylenedipyridine molecules, were reacted under compressed CO<inf>2</inf> at 60 °C and 20 MPa for periods of 4 or 24 h. The success achieved in the synthesis of the different studied 1D-MOFs was related to the solubility of the reagents in supercritical CO<inf>2</inf>. The reaction yield of the synthesized coordination polymers via the supercritical route was close to 100% because both the reactants were almost completely depleted in the performed experiments. © The Royal Society of Chemistry 2015. | - |
dc.description.sponsorship | This work was partially financed by EU COST project MP1202 OC-2011-2-10820 and by the Generalitat de Catalunya 2014SGR377. A. López-Periago acknowledges the RyC-2012- 11588 contract. We acknowledge support by the CSIC Open Access Publication Initiative through its Unit of Information Resources for Research (URICI) | - |
dc.publisher | Royal Society of Chemistry (UK) | - |
dc.relation.isversionof | Publisher's version | - |
dc.rights | openAccess | - |
dc.title | Exploring a novel preparation method of 1D metal organic frameworks based on supercritical CO2 | - |
dc.type | artículo | - |
dc.identifier.doi | 10.1039/c5dt00521c | - |
dc.relation.publisherversion | http://dx.doi.org/10.1039/c5dt00521c | - |
dc.date.updated | 2016-10-04T10:27:24Z | - |
dc.description.version | Peer Reviewed | - |
dc.language.rfc3066 | eng | - |
dc.rights.license | http://creativecommons.org/licenses/by-nc/4.0 | - |
dc.contributor.funder | CSIC - Unidad de Recursos de Información Científica para la Investigación (URICI) | - |
dc.contributor.funder | Ministerio de Economía y Competitividad (España) | - |
dc.contributor.funder | Generalitat de Catalunya | - |
dc.contributor.funder | European Commission | - |
dc.relation.csic | Sí | - |
dc.identifier.funder | http://dx.doi.org/10.13039/501100003329 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100002809 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100000780 | es_ES |
dc.type.coar | http://purl.org/coar/resource_type/c_6501 | es_ES |
item.openairecristype | http://purl.org/coar/resource_type/c_18cf | - |
item.fulltext | With Fulltext | - |
item.cerifentitytype | Publications | - |
item.openairetype | artículo | - |
item.grantfulltext | open | - |
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