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Hydrogen capture by porphyrins at the TiO2(110) surface

AuthorsLovat, Giacomo; Abadia, Mikel; Rogero, Celia CSIC ORCID; Vittadini, Andrea; Floreano, Luca
Issue Date2015
PublisherRoyal Society of Chemistry (UK)
CitationPhysical Chemistry Chemical Physics 17(44): 30119-30124 (2015)
AbstractMetal-free porphyrin molecules adsorb on the rutile TiO(110) surface with their pyrrolic nitrogen atoms atop the O-bridge rows, whereas the iminic nitrogen atoms capture two additional hydrogen atoms. Hydrogenation occurs spontaneously at room temperature, irrespective of the distance of the polypyrrolic macrocycle from the surface, as varied by changing the porphyrin functionalization.
Identifiersdoi: 10.1039/C5CP05437K
issn: 1463-9076
e-issn: 1463-9084
Appears in Collections:(CFM) Artículos
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