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Título

The role of Au, Cu & CeO2 and their interactions for an enhanced WGS performance

AutorReina, T.R. ; Ivanova, Svetlana ; Centeno, Miguel Ángel ; Odriozola, José Antonio
Palabras claveWGS
Gold catalysts
Cerium oxide
Copper oxide
Fecha de publicación2016
EditorElsevier
CitaciónApplied Catalysis B - Environmental, 187: 98-107 (2016)
ResumenThe WGS reaction over multicomponent Au/Ce1-xCuxO2/Al2O3 catalysts is studied in this work. The systems are carefully designed aiming to take advantage of every active phase included in the formulation: gold, ceria and copper. Special emphasis is given to the CeO2-CuO synergy and its influence on the displayed catalytic performance with and without gold. To this aim a meaningful correlation between the physicochemical properties of the mixed materials and their activity/stability is proposed. In general terms the developed catalysts present high activity under realistic WGS reaction conditions, with fairly good long term stability. In addition, the systems successfully withstand start-up/shut-downs situations, indispensable requisite for real applications in the field of pure hydrogen production for fuel cell goals.
Versión del editorhttp://dx.doi.org/10.1016/j.apcatb.2016.01.031
URIhttp://hdl.handle.net/10261/128668
DOI10.1016/j.apcatb.2016.01.031
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