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Campo DC | Valor | Lengua/Idioma |
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dc.contributor.author | Yan, Geng | - |
dc.contributor.author | Pfattner, Raphael | - |
dc.contributor.author | Campos García, Antonio | - |
dc.contributor.author | Wei, Wang | - |
dc.contributor.author | Jeannin, Olivier | - |
dc.contributor.author | Hauser, Jürg | - |
dc.contributor.author | Puigdollers-González, Joaquim | - |
dc.contributor.author | Bromley, Stefan T. | - |
dc.contributor.author | Decurtins, Silvio | - |
dc.contributor.author | Veciana, Jaume | - |
dc.contributor.author | Rovira, Concepció | - |
dc.contributor.author | Mas Torrent, Marta | - |
dc.contributor.author | Shi-Xia, Liu | - |
dc.date.accessioned | 2015-07-01T11:50:18Z | - |
dc.date.available | 2015-07-01T11:50:18Z | - |
dc.date.issued | 2014-08-12 | - |
dc.identifier.citation | Chemistry - a European Journal 20(50):16672-16679 (2014) | es_ES |
dc.identifier.issn | 0947-6539 | - |
dc.identifier.uri | http://hdl.handle.net/10261/117434 | - |
dc.description.abstract | Three new organic semiconductors, in which either two methoxy units are directly linked to a dibenzotetrathiafulvalene (DB-TTF) central core and a 2,1,3-chalcogendiazole is fused on the one side, or four methoxy groups are linked to the DB-TTF, have been synthesised as active materials for organic field-effect transistors (OFETs). Their electrochemical behaviour, electronic absorption and fluorescence emission as well as photoinduced intramolecular charge transfer were studied. The electron-withdrawing 2,1,3-chalcogendiazole unit significantly affects the electronic properties of these semiconductors, lowering both the HOMO and LUMO energy levels and hence increasing the stability of the semiconducting material. The solution-processed single-crystal transistors exhibit high performance with a hole mobility up to 0.04 cm2 V−1 s−1 as well as good ambient stability. | es_ES |
dc.description.sponsorship | Financial support for this research by the Swiss National Science Foundation (Grant No. 200021–147143), ERC StG 2012– 306826 e-GAMES, the Networking Research Center on Bioengineering, Biomaterials and Nanomedicine (CIBER-BBN), the DGI (Spain) with project BE-WELL CTQ2013–40480-R, TEC2011– 27859-C02–01, and MAT2012–30924, the Generalitat de Catalunya with project 2014-SGR-17, as well as by the National Natural Science Foundation of China (No. 21175077) | es_ES |
dc.language.iso | eng | es_ES |
dc.publisher | Wiley-VCH | es_ES |
dc.relation.isversionof | Postprint | es_ES |
dc.rights | openAccess | en_EN |
dc.subject | Donor–acceptor | es_ES |
dc.subject | systems | es_ES |
dc.subject | Fused-ring | es_ES |
dc.subject | systems | es_ES |
dc.subject | Molecular | es_ES |
dc.subject | electronics | es_ES |
dc.subject | Semiconductors | es_ES |
dc.subject | Thin | es_ES |
dc.subject | films | es_ES |
dc.title | HOMO Stabilisation in p-Extended Dibenzotetrathiafulvalene Derivatives for Their Application in Organic Field-Effect Transistors | es_ES |
dc.type | artículo | es_ES |
dc.description.peerreviewed | Peer reviewed | es_ES |
dc.relation.publisherversion | http://onlinelibrary.wiley.com/doi/10.1002/chem.201404508/epdf | es_ES |
dc.embargo.terms | 2015-08-12 | es_ES |
dc.relation.csic | Sí | es_ES |
dc.type.coar | http://purl.org/coar/resource_type/c_6501 | es_ES |
item.openairetype | artículo | - |
item.grantfulltext | open | - |
item.cerifentitytype | Publications | - |
item.openairecristype | http://purl.org/coar/resource_type/c_18cf | - |
item.fulltext | With Fulltext | - |
item.languageiso639-1 | en | - |
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YanGeng-ChemEurJ-2014-postprint.pdf | 445,6 kB | Adobe PDF | Visualizar/Abrir |
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