Please use this identifier to cite or link to this item: http://hdl.handle.net/10261/10355
Share/Export:
logo share SHARE logo core CORE BASE
Visualizar otros formatos: MARC | Dublin Core | RDF | ORE | MODS | METS | DIDL | DATACITE
Title

Altitudinal gradients of PBDEs and PCBs in fish from European high mountain lakes

AuthorsGallego, Eva; Grimalt, Joan O. CSIC ORCID ; Bartrons, Mireia CSIC ORCID; López Fernández, Jordi F. CSIC; Camarero, Lluís ; Catalán, Jordi; Stuchlík, Evzen; Battarbee, Rick
KeywordsPolybromodiphenyl ethers (PBDEs)
Polychlorobiphenyls (PCBs)
Compound concentration
Lower temperatures
Global distillation model
Issue Date6-Mar-2007
PublisherAmerican Chemical Society
CitationEnvironmental Science & Technology 41(7): 2196-2202 (2007)
AbstractA first case of temperature-dependent distribution of polybromodiphenyl ethers (PBDEs) in remote areas is shown. Analysis of these compounds in fish from Pyrenean lakes distributed along an altitudinal transect shows higher concentrations at lower temperatures, as predicted in the global distillation model. Conversely, no temperature-dependent distribution is observed in a similar transect in the Tatra mountains (Central Europe) nor in fish from high mountain lakes distributed throughout Europe. The fish concentrations of polychlorobiphenyls (PCBs) examined for comparison showed significant temperature correlations in all these studied lakes. Cold trapping of both PCBs and PBDEs concerned the less volatile congeners. In the Pyrenean lake transect the concentrations of PCBs and PBDEs in fish were correlated despite the distinct use of these compounds and their 40 year time lag of emissions to the environment. Thus, temperature effects have overcome these anthropogenic differences constituting at present the main process determining their distributions. These cases of distinct PBDEs and PCBs behavior in high mountains likely reflect early stages in the environmental distribution of the former since they have been under secondary redistribution processes over much shorter time than the latter.
Description7 pages, 4 figures.-- PMID: 17438763 [PubMed].-- Printed version published on Apr 1, 2007.
Supplementary information (Materials and methods, Suppl. figure S1, tables S1-S4, 9 pages) available at: http://pubs.acs.org/doi/suppl/10.1021/es062197m/suppl_file/es062197msi20061218_033001.pdf
Publisher version (URL)http://dx.doi.org/10.1021/es062197m
URIhttp://hdl.handle.net/10261/10355
DOI10.1021/es062197m
ISSN0013-936x
E-ISSN1520-5851
Appears in Collections:(IDAEA) Artículos
(CEAB) Artículos

Show full item record
Review this work

SCOPUSTM   
Citations

60
checked on Jan 22, 2022

WEB OF SCIENCETM
Citations

55
checked on Jan 16, 2022

Page view(s)

463
checked on Jan 22, 2022

Google ScholarTM

Check

Altmetric

Dimensions


WARNING: Items in Digital.CSIC are protected by copyright, with all rights reserved, unless otherwise indicated.