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http://hdl.handle.net/10261/102114
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dc.contributor.author | Pérez-Baena, Irma | - |
dc.contributor.author | Barroso-Bujans, Fabienne | - |
dc.contributor.author | Gasser, Urs | - |
dc.contributor.author | Arbe, Arantxa | - |
dc.contributor.author | Moreno Segurado, Ángel J. | - |
dc.contributor.author | Colmenero de León, Juan | - |
dc.contributor.author | Pomposo, José A. | - |
dc.date.accessioned | 2014-09-15T13:00:55Z | - |
dc.date.available | 2014-09-15T13:00:55Z | - |
dc.date.issued | 2013 | - |
dc.identifier | doi: 10.1021/mz4003744 | - |
dc.identifier | e-issn: 2161-1653 | - |
dc.identifier.citation | ACS Macro Letters 2(9): 775-779 (2013) | - |
dc.identifier.uri | http://hdl.handle.net/10261/102114 | - |
dc.description.abstract | The development of simple, efficient, and robust strategies affording the facile construction of biomimetic organocatalytic nano-objects is currently a subject of great interest. Herein, a new pathway to artificial organocatalysts based on partially collapsed individual soft nano-objects displaying useful and diverse biomimetic catalytic functions is reported. Single-chain polymer nanoparticles endowed with enzyme-mimetic activity synthesized following this new route display (i) a relatively extended morphology under good solvent conditions, as revealed by small angle neutron scattering and coarse-grained molecular dynamics simulation results, (ii) multiple, compartmentalized, and accessible catalytic sites in which borane catalytic units are retained via B···O interactions, and (iii) unprecedented reductase and polymerase enzyme-mimetic properties. © 2013 American Chemical Society. | - |
dc.description.sponsorship | Financial support from the projects MAT2012-31088 (MINECO) and IT-654-13 (GV) is acknowledged. I. P.-B. acknowledges CSIC for her JAE-PREDOC grant. This work is based on has been supported by the European Commission under the 7th Framework Programme through the 'Research Infrastructures' action of the 'Capacities' Programme, NMI3-II Grant number 283883. | - |
dc.publisher | American Chemical Society | - |
dc.relation | info:eu-repo/grantAgreement/EC/FP7/283883 | - |
dc.relation.isversionof | Postprint | - |
dc.rights | openAccess | - |
dc.title | Endowing single-chain polymer nanoparticles with enzyme-mimetic activity | - |
dc.type | artículo | - |
dc.identifier.doi | 10.1021/mz4003744 | - |
dc.relation.publisherversion | http://dx.doi.org/10.1021/mz4003744 | - |
dc.date.updated | 2014-09-15T13:00:56Z | - |
dc.description.version | Peer Reviewed | - |
dc.language.rfc3066 | eng | - |
dc.contributor.funder | European Commission | - |
dc.contributor.funder | Ministerio de Economía y Competitividad (España) | - |
dc.contributor.funder | Eusko Jaurlaritza | - |
dc.contributor.funder | Consejo Superior de Investigaciones Científicas (España) | - |
dc.identifier.funder | http://dx.doi.org/10.13039/501100000780 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100003329 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100003339 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100003086 | es_ES |
dc.type.coar | http://purl.org/coar/resource_type/c_6501 | es_ES |
item.openairetype | artículo | - |
item.grantfulltext | open | - |
item.cerifentitytype | Publications | - |
item.openairecristype | http://purl.org/coar/resource_type/c_18cf | - |
item.fulltext | With Fulltext | - |
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Endowing single-chain.pdf | 761,21 kB | Adobe PDF | Visualizar/Abrir |
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