2024-03-29T10:39:26Zhttp://digital.csic.es/dspace-oai/requestoai:digital.csic.es:10261/1893972021-12-27T16:43:23Zcom_10261_89com_10261_3col_10261_342
DIGITAL.CSIC
author
Chiodini, Stefano
author
Reinares-Fisac, Daniel
author
Espinosa, Francisco M.
author
Gutiérrez-Puebla, Enrique
author
Monge, M. Ángeles
author
Gándara Barragán, Felipe
author
García García, Ricardo
funder
Ministerio de Economía y Competitividad (España)
funder
European Research Council
2019-08-29T09:19:26Z
2019-08-29T09:19:26Z
2017-09-11
Scientific Reports 7: 11088 (2017)
http://hdl.handle.net/10261/189397
10.1038/s41598-017-11479-4
http://dx.doi.org/10.13039/501100000781http://dx.doi.org/10.13039/501100003329
28894192
Metal-organic frameworks (MOFs) are a class of crystalline materials with a variety of applications in gas storage, catalysis, drug delivery or light harvesting. The optimization of those applications requires the characterization of MOF structure in the relevant environment. Dynamic force microscopy has been applied to follow dynamic processes of metal-organic-framework material. We provide images with spatial and time resolutions, respectively, of angstrom and seconds that show that Ce-RPF-8 surfaces immersed in water and glycerol experience a surface reconstruction process that is characterized by the diffusion of the molecular species along the step edges of the open terraces. The rate of the surface reconstruction process depends on the liquid. In water it happens spontaneously while in glycerol is triggered by applying an external force.
eng
openAccess
Angstrom-resolved metal-organic framework-liquid interfaces
artículo
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URL
https://digital.csic.es/bitstream/10261/189397/1/angstrom-resolved_metal-organic_framework-liquid_interfaces.pdf
File
MD5
01a07ddc9fe5d42d3d098265217d607c
1852196
application/pdf
angstrom-resolved_metal-organic_framework-liquid_interfaces.pdf