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Title

Design of a bifunctional Ir-Zr based metal-organic framework heterogeneous catalyst for the N-alkylation of amines with alcohols

AuthorsRasero-Almansa, Antonia M.; Corma, Avelino; Iglesias, Marta ; Sánchez, Félix
KeywordsBifunctional catalyst
Heterogeneous catalyst
Iridium
N-alkylation
Zr-based MOF
Issue Date2014
CitationChemCatChem 6 : 1794-1800 (2014)
AbstractThe direct N-alkylation of amines with alcohols was performed with an Ir-Zr-based metal-organic framework multifunctional heterogeneous catalyst. This system is efficient and environmentally benign for the synthesis of various organic amines in air in the absence of a base. The catalyst was recovered and reused without significant loss of activity, and only water was produced as a byproduct. Better be direct than elusive: The direct N-alkylation of amines with alcohols is performed with an Ir-Zr-based metal-organic framework multifunctional heterogeneous catalyst. This system is efficient and environmentally benign for the synthesis of various organic amines in air in the absence of a base. The catalyst is recovered and reused without significant loss of activity, and only water is produced as a byproduct.
URIhttp://hdl.handle.net/10261/99365
DOI10.1002/cctc.201402101
Identifiersdoi: 10.1002/cctc.201402101
issn: 1867-3880
e-issn: 1867-3899
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