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Title

Generalized Chudley-Elliott vibration-jump model in activated atom surface diffusion

AuthorsMartínez Casado, R. CSIC; Vega, J. L.; Sanz, Ángel S. CSIC ORCID; Miret-Artés, Salvador CSIC ORCID
Issue DateMay-2007
PublisherAmerican Institute of Physics
CitationJournal of Chemical Physics 126(19): 194711 (2007)
AbstractHere the authors provide a generalized Chudley-Elliott expression for the activated atom surface diffusion which takes into account the coupling between both low-frequency vibrational motion (namely, the frustrated translational modes) and diffusion. This expression is derived within the Gaussian approximation framework for the intermediate scattering function at low coverage. Moreover, inelastic contributions (arising from creation and annihilation processes) to the full width at half maximum of the quasielastic peak are also obtained.
Description5 pages, 2 figures.
Publisher version (URL)http://dx.doi.org/10.1063/1.2735586
URIhttp://hdl.handle.net/10261/22345
DOI10.1063/1.2735586
ISSN0021-9606
Appears in Collections:(CFMAC-IFF) Artículos




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