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Título: | Purely armchair or partially chiral: noncontact atomic force microscopy characterization of dibromo-bianthryl-based graphene nanoribbons grown on Cu(111) |
Autor: | Sánchez-Sánchez, Carlos CSIC ORCID ; Dienel, Thomas; Deniz, Okan; Ruffieux, Pascal; Berger, Reinhard; Feng, Xinliang; Müllen, Klaus; Fasel, Román | Palabras clave: | Functionalized tip Bottom-up On-surface synthesis Armchair Chiral Graphene nanoribbons |
Fecha de publicación: | 23-ago-2016 | Editor: | American Chemical Society | Citación: | ACS Nano 10(8): 8006-8011 (2016) | Resumen: | We report on the atomic structure of graphene nanoribbons (GNRs) formed via on-surface synthesis from 10,10′-dibromo-9,9′-bianthryl (DBBA) precursors on Cu(111). By means of ultrahigh vacuum noncontact atomic force microscopy with CO-functionalized tips we unveil the chiral nature of the so-formed GNRs, a structure that has been under considerable debate. Furthermore, we prove that - in this particular case - the coupling selectivity usually introduced by halogen substitution is overruled by the structural and catalytic properties of the substrate. Specifically, we show that identical chiral GNRs are obtained from 9,9′-bianthryl, the unsubstituted sister molecule of DBBA. | Versión del editor: | https://doi.org/10.1021/acsnano.6b04025 | URI: | http://hdl.handle.net/10261/185804 | DOI: | 10.1021/acsnano.6b04025 | Identificadores: | doi: 10.1021/acsnano.6b04025 e-issn: 1936-086X issn: 1936-0851 |
Aparece en las colecciones: | (ICMM) Artículos |
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