Please use this identifier to cite or link to this item: http://hdl.handle.net/10261/16527
Share/Export:
logo share SHARE logo core CORE BASE
Visualizar otros formatos: MARC | Dublin Core | RDF | ORE | MODS | METS | DIDL | DATACITE
Title

Atmospheric concentrations and deposition of polychorinated biphenyls to the Hudson River Estuary

AuthorsTotten, Lisa A.; Gigliotti, Cari L.; VanRy, Daryl A.; Offenberg, John H.; Nelson, Eric D.; Dachs, Jordi CSIC ORCID; Reinfelder, John R.; Eisenreich, Steven J.
KeywordsPolychlorinated biphenyls
PCBs
Atmospheric concentrations
Atmospheric deposition
Hudson River Estuary
Issue Date25-Mar-2004
PublisherAmerican Chemical Society
CitationEnvironmental Science and Technology 38(9): 2568-2573 (2004)
AbstractThe first estimates of atmospheric deposition fluxes of polychlorinated biphenyls (PCBs) to the Hudson River Estuary are presented. Concentrations of PCBs were measured in air, aerosol, and precipitation at nine sites representing a variety of land-use regimes at regular intervals from October 1997 through May 2001. Highest concentrations in the gas phase were observed at urban sites such as Camden and Jersey City (∑PCB concentrations averaged 3250 and 1260 pg m-3, respectively). In great portions of the state encompassing forested, coastal, and suburban environments, gas-phase ∑PCB concentrations were essentially the same (averaging 150−220 pg m-3). This spatial trend suggests that atmospheric PCBs arise from highly localized, urban sources which influence atmospheric concentrations and deposition fluxes over a distance of a few tens of kilometers. Atmospheric ∑PCB deposition fluxes (gas absorption + dry particle deposition + wet deposition) ranged from 7.3 to 340 μg m-2 yr-1 and increased with proximity to urban areas. While the magnitude of the fluxes increased with urbanization, the relative proportions of wet, dry, and gaseous deposition remained largely constant. Because the Hudson River Estuary is adjacent to urban areas such as Jersey City, it is subject to higher depositional fluxes of PCBs. These depositional fluxes are at least 2−10 times those estimated for the Chesapeake Bay and Lake Michigan. Inputs of PCBs to the Hudson River Estuary from the upper Hudson River and from wastewater treatment plants are 8−18 times atmospheric inputs, and volatilization of PCBs from the estuary exceeds atmospheric deposition of low molecular weight PCBs.
Description6 pages, 3 figures, 1 table.-- PMID: 15180052 [PubMed].-- Printed version published May 1, 2004.-- Supporting information available at: http://pubs.acs.org/doi/suppl/10.1021/es034878c
Publisher version (URL)http://dx.doi.org/10.1021/es034878c
URIhttp://hdl.handle.net/10261/16527
DOI10.1021/es034878c
ISSN0013-936X
Appears in Collections:(IDAEA) Artículos

Show full item record
Review this work

SCOPUSTM   
Citations

64
checked on May 22, 2022

WEB OF SCIENCETM
Citations

58
checked on May 24, 2022

Page view(s)

350
checked on May 27, 2022

Google ScholarTM

Check

Altmetric

Dimensions


WARNING: Items in Digital.CSIC are protected by copyright, with all rights reserved, unless otherwise indicated.