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Campo DC | Valor | Lengua/Idioma |
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dc.contributor.author | Palacio, Irene | es_ES |
dc.contributor.author | Pinardi, Anna Lisa | es_ES |
dc.contributor.author | Martínez, José I. | es_ES |
dc.contributor.author | Preobrajenski, Alexei | es_ES |
dc.contributor.author | Cossaro, Albano | es_ES |
dc.contributor.author | Jancarik, Andrej | es_ES |
dc.contributor.author | Stará̈, Irena G. | es_ES |
dc.contributor.author | Méndez, Javier | es_ES |
dc.contributor.author | Martín-Gago, José A. | es_ES |
dc.contributor.author | López, María Francisca | es_ES |
dc.date.accessioned | 2018-04-26T12:36:09Z | - |
dc.date.available | 2018-04-26T12:36:09Z | - |
dc.date.issued | 2017-07-31 | - |
dc.identifier.citation | Physical Chemistry Chemical Physics 19: 22454-22461 (2017) | es_ES |
dc.identifier.issn | 1463-9076 | - |
dc.identifier.uri | http://hdl.handle.net/10261/164246 | - |
dc.description.abstract | New nanoarchitectures can be built from polycyclic aromatic hydrocarbons (PAHs) by exploiting the capability of some metal surfaces for inducing cyclodehydrogenation reactions. This bottom-up approach allows the formation of nanostructures with a different dimensionality from the same precursor as a consequence of the diffusion and coupling of the PAHs adsorbed on the surface. In this work we present a thorough study, by means of a combination of X-ray photoemission spectroscopy, near-edge X-ray absorption fine structure and scanning tunneling microscopy with first principle calculations of the structural and chemical transformations undergone by pyridyl-substituted dibenzo[5]helicene on three coinage surfaces, namely Cu(110), Cu(111) and Au(111). Upon annealing, on-surface chemical reactions are promoted affecting the adsorbate/substrate and the molecule/molecule interactions. This thermally induced process favours the transformation from diffusing isolated molecules to polymeric nanographene chains and finally to N-doped graphene. | es_ES |
dc.description.sponsorship | This work has been supported by the Spanish MINECO (Grant MAT2014-54231-C04-1-P), the EU via the ERC-Synergy Program (Grant ERC-2013-SYG-610256 NANOCOSMOS) and the Innovation program under grant agreement No. 696656 (GrapheneCore1-Graphene-based disruptive technologies). JIM acknowledges the financial support by the “Ramón y Cajal” Program of MINECO (Grant RYC-2015-17730) and Nanocosmos, as well as computing resources from CTI-CSIC. | es_ES |
dc.language.iso | eng | es_ES |
dc.publisher | Royal Society of Chemistry (UK) | es_ES |
dc.relation | info:eu-repo/grantAgreement/MINECO/Plan Estatal de Investigación Científica y Técnica y de Innovación 2013-2016/MAT2014-54231-C04-1-P | es_ES |
dc.relation | info:eu-repo/grantAgreement/EC/FP7/610256 | es_ES |
dc.relation | info:eu-repo/grantAgreement/EC/FP7/696656 | es_ES |
dc.relation | info:eu-repo/grantAgreement/MINECO/Plan Estatal de Investigación Científica y Técnica y de Innovación 2013-2016/RYC-2015-17730 | es_ES |
dc.relation.isversionof | Postprint | - |
dc.rights | openAccess | en_EN |
dc.title | Spectroscopic characterization of the on-surface induced (cyclo)dehydrogenation of a N-heteroaromatic compound on noble metal surfaces | es_ES |
dc.type | artículo | es_ES |
dc.identifier.doi | 10.1039/C7CP03955G | - |
dc.description.peerreviewed | Peer reviewed | es_ES |
dc.relation.publisherversion | http://dx.doi.org/10.1039/C7CP03955G | es_ES |
dc.identifier.e-issn | 1463-9084 | - |
dc.contributor.funder | Ministerio de Economía y Competitividad (España) | es_ES |
dc.contributor.funder | European Commission | es_ES |
dc.contributor.funder | European Research Council | es_ES |
dc.relation.csic | Sí | es_ES |
oprm.item.hasRevision | no ko 0 false | * |
dc.identifier.funder | http://dx.doi.org/10.13039/501100000780 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100003329 | es_ES |
dc.identifier.funder | http://dx.doi.org/10.13039/501100000781 | es_ES |
dc.type.coar | http://purl.org/coar/resource_type/c_6501 | es_ES |
item.openairetype | artículo | - |
item.grantfulltext | open | - |
item.cerifentitytype | Publications | - |
item.openairecristype | http://purl.org/coar/resource_type/c_18cf | - |
item.fulltext | With Fulltext | - |
item.languageiso639-1 | en | - |
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IPalacio_PCCP2017.pdf | 956,96 kB | Adobe PDF | Visualizar/Abrir |
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