Por favor, use este identificador para citar o enlazar a este item:
http://hdl.handle.net/10261/15353
COMPARTIR / EXPORTAR:
SHARE CORE BASE | |
Visualizar otros formatos: MARC | Dublin Core | RDF | ORE | MODS | METS | DIDL | DATACITE | |
Título: | Atmospheric dry deposition of persistent organic pollutants to the Atlantic and inferences for the global oceans |
Autor: | Jurado, Elena CSIC ORCID; Jaward, Foday M.; Lohmann, Rainer; Jones, Kevin C.; Simó, Rafel CSIC ORCID ; Dachs, Jordi CSIC ORCID | Fecha de publicación: | 29-sep-2004 | Editor: | American Chemical Society | Citación: | Environmental Science and Technology 38(21): 5505-5513 (2004) | Resumen: | Atmospheric deposition to the oceans is a key process affecting the global dynamics and sinks of persistent organic pollutants (POPs). A new methodology that combines aerosol remote sensing measurements with measured POP aerosol-phase concentrations is presented to derive dry particulate depositional fluxes of POPs to the oceans. These fluxes are compared with those due to diffusive air−water exchange. For all polychlorinated biphenyl (PCB) congeners and lower chlorinated dibenzo-p-dioxins and furans (PCDD/Fs), air−water exchange dominates the dry deposition mechanism. However, this tendency reverses in some areas, such as in marine aerosol influenced areas and dust outflow regions, consistent with the important variability encountered for the depositional fluxes. Seasonal variability is mainly found in mid-high latitudes, due to the important influence of wind speed enhancing dry deposition fluxes and temperature as a driver of the gas-particle partitioning of POPs. The average dry aerosol deposition flux of ΣPCBs and ΣPCDD/Fs to the Atlantic Ocean is calculated to be in the order of 66 ng m-2 yr-1 and 9 ng m-2 yr-1 respectively. The total dry aerosol deposition of ∑PCBs and ∑PCDD/Fs to the Atlantic Ocean is estimated to be 2200 kg yr-1 and 500 kg yr-1, respectively, while the net air−water exchange is higher, 22000 kg ∑PCBs yr-1 for PCBs and 1300 kg ∑PCDD/Fs yr-1. Furthermore, it is suggested that marine aerosol plays an important role in scavenging atmospheric contaminants | Descripción: | 9 pages, 6 figures, 1 table.-- PMID: 15575265 [PubMed] Supporting information available: Further details on cruise data and methodology to estimate dry deposition velocities (Annexes I, II, and III) and comparison of gross gaseous absorption and dry aerosol deposition fluxes (Annex IV).-- Available at: http://pubs.acs.org/doi/suppl/10.1021/es049240v |
Versión del editor: | https://doi.org/10.1021/es049240v | URI: | http://hdl.handle.net/10261/15353 | DOI: | 10.1021/es049240v | ISSN: | 0013-936X |
Aparece en las colecciones: | (IDAEA) Artículos (ICM) Artículos |
Mostrar el registro completo
CORE Recommender
SCOPUSTM
Citations
135
checked on 18-abr-2024
WEB OF SCIENCETM
Citations
128
checked on 29-feb-2024
Page view(s)
456
checked on 24-abr-2024
Google ScholarTM
Check
Altmetric
Altmetric
NOTA: Los ítems de Digital.CSIC están protegidos por copyright, con todos los derechos reservados, a menos que se indique lo contrario.