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Título

Spin-phonon coupling in epitaxial Sr0.6Ba0.4MnO3 thin films

AutorGoian, V.; Langenberg, Eric CSIC ORCID; Marcano, N. CSIC ORCID; Bovtun, V.; Maurel, Laura; Kempa, M.; Prokscha, Thomas; Algarabel, Pedro A. CSIC ORCID; Pardo, J. A. CSIC ORCID; Kamba, S.
Fecha de publicación2017
EditorAmerican Physical Society
CitaciónPhysical Review B 95(7): 075126 (2017)
ResumenSpin-phonon coupling is investigated in epitaxially strained Sr1-xBaxMnO3 thin films with perovskite structure by means of microwave (MW) and infrared (IR) spectroscopy. In this work we focus on the Sr0.6Ba0.4MnO3 composition grown on (LaAlO3)0.3(Sr2AlTaO6)0.7 substrate. The MW complex electromagnetic response shows a decrease in the real part and a clear anomaly in the imaginary part around 150 K. Moreover, it coincides with a 17% hardening of the lowest-frequency polar phonon seen in IR reflectance spectra. In order to further elucidate this phenomenon, low-energy muon-spin spectroscopy was carried out, signaling the emergence of antiferromagnetic order with Néel temperature (TN) around 150 K. Thus, our results confirm that epitaxial Sr0.6Ba0.4MnO3 thin films display strong spin-phonon coupling below TN, which may stimulate further research on tuning the magnetoelectric coupling by controlling the epitaxial strain and chemical pressure in the Sr1-xBaxMnO3 system.
DescripciónUnder the terms of the Creative Commons Attribution license.-- et al.
Versión del editorhttps://doi.org/10.1103/PhysRevB.95.075126
URIhttp://hdl.handle.net/10261/148733
DOI10.1103/PhysRevB.95.075126
Identificadoresdoi: 10.1103/PhysRevB.95.075126
issn: 2469-9950
e-issn: 2469-9969
Aparece en las colecciones: (ICMA) Artículos




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